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<!DOCTYPE article PUBLIC "-//NLM//DTD JATS (Z39.96) Journal Publishing DTD with OASIS Tables with MathML3 v1.2 20190208//EN" "JATS-journalpublishing-oasis-article1-mathml3.dtd">
<article article-type="research-article" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" xmlns:oasis="http://www.niso.org/standards/z39-96/ns/oasis-exchange/table"><front><journal-meta><journal-id journal-id-type="publisher-id">PRL</journal-id><journal-id journal-id-type="coden">PRLTAO</journal-id><journal-title-group><journal-title>Physical Review Letters</journal-title><abbrev-journal-title>Phys. Rev. Lett.</abbrev-journal-title></journal-title-group><issn pub-type="ppub">0031-9007</issn><issn pub-type="epub">1079-7114</issn><publisher><publisher-name>American Physical Society</publisher-name></publisher></journal-meta><article-meta><article-id pub-id-type="doi">10.1103/PhysRevLett.123.221802</article-id><article-categories><subj-group subj-group-type="toc-major"><subject>LETTERS</subject></subj-group><subj-group subj-group-type="toc-minor"><subject>Elementary Particles and Fields</subject></subj-group></article-categories><title-group><article-title>Improved Upper Limit on the Neutrino Mass from a Direct Kinematic Method by KATRIN</article-title></title-group><contrib-group><contrib contrib-type="author"><name><surname>Aker</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Altenmüller</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a10 a3 a4"><sup>10,3,4</sup></xref></contrib><contrib contrib-type="author"><name><surname>Arenz</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a5"><sup>5</sup></xref></contrib><contrib contrib-type="author"><name><surname>Babutzka</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Barrett</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a7"><sup>7</sup></xref></contrib><contrib contrib-type="author"><name><surname>Bauer</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Beck</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a8 a12"><sup>8,12</sup></xref></contrib><contrib contrib-type="author"><name><surname>Beglarian</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Behrens</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a6 a1 a8"><sup>6,1,8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Bergmann</surname><given-names>T.</given-names></name><xref ref-type="aff" rid="a10 a3 a9"><sup>10,3,9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Besserer</surname><given-names>U.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Blaum</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a11"><sup>11</sup></xref></contrib><contrib contrib-type="author"><name><surname>Block</surname><given-names>F.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Bobien</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a2"><sup>2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Bokeloh</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref><xref ref-type="author-notes" rid="n4"><sup>§</sup></xref></contrib><contrib contrib-type="author"><name><surname>Bonn</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a12"><sup>12</sup></xref><xref ref-type="author-notes" rid="n1"><sup>,*</sup></xref></contrib><contrib contrib-type="author"><name><surname>Bornschein</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Bornschein</surname><given-names>L.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Bouquet</surname><given-names>H.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Brunst</surname><given-names>T.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Caldwell</surname><given-names>T. S.</given-names></name><xref ref-type="aff" rid="a13 a14"><sup>13,14</sup></xref></contrib><contrib contrib-type="author"><name><surname>La Cascio</surname><given-names>L.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Chilingaryan</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Choi</surname><given-names>W.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Corona</surname><given-names>T. J.</given-names></name><xref ref-type="aff" rid="a13 a14 a7"><sup>13,14,7</sup></xref></contrib><contrib contrib-type="author"><name><surname>Debowski</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a15 a6"><sup>15,6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Deffert</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Descher</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Doe</surname><given-names>P. J.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Dragoun</surname><given-names>O.</given-names></name><xref ref-type="aff" rid="a17"><sup>17</sup></xref></contrib><contrib contrib-type="author"><name><surname>Drexlin</surname><given-names>G.</given-names></name><xref ref-type="aff" rid="a6 a1"><sup>6,1</sup></xref><xref ref-type="author-notes" rid="n2"><sup>†</sup></xref></contrib><contrib contrib-type="author"><name><surname>Dunmore</surname><given-names>J. A.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Dyba</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Edzards</surname><given-names>F.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Eisenblätter</surname><given-names>L.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Eitel</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Ellinger</surname><given-names>E.</given-names></name><xref ref-type="aff" rid="a15"><sup>15</sup></xref></contrib><contrib contrib-type="author"><name><surname>Engel</surname><given-names>R.</given-names></name><xref ref-type="aff" rid="a1 a6"><sup>1,6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Enomoto</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Erhard</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Eversheim</surname><given-names>D.</given-names></name><xref ref-type="aff" rid="a5"><sup>5</sup></xref></contrib><contrib contrib-type="author"><name><surname>Fedkevych</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Felden</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Fischer</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Flatt</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a12"><sup>12</sup></xref></contrib><contrib contrib-type="author"><name><surname>Formaggio</surname><given-names>J. A.</given-names></name><xref ref-type="aff" rid="a7"><sup>7</sup></xref></contrib><contrib contrib-type="author"><name><surname>Fränkle</surname><given-names>F. M.</given-names></name><xref ref-type="aff" rid="a1 a13 a14"><sup>1,13,14</sup></xref></contrib><contrib contrib-type="author"><name><surname>Franklin</surname><given-names>G. B.</given-names></name><xref ref-type="aff" rid="a18"><sup>18</sup></xref></contrib><contrib contrib-type="author"><name><surname>Frankrone</surname><given-names>H.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Friedel</surname><given-names>F.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Fuchs</surname><given-names>D.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Fulst</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Furse</surname><given-names>D.</given-names></name><xref ref-type="aff" rid="a7"><sup>7</sup></xref></contrib><contrib contrib-type="author"><name><surname>Gauda</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Gemmeke</surname><given-names>H.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Gil</surname><given-names>W.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Glück</surname><given-names>F.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Görhardt</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Groh</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Grohmann</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a2"><sup>2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Grössle</surname><given-names>R.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Gumbsheimer</surname><given-names>R.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Ha Minh</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Hackenjos</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a1 a2 a6"><sup>1,2,6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Hannen</surname><given-names>V.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Harms</surname><given-names>F.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Hartmann</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Haußmann</surname><given-names>N.</given-names></name><xref ref-type="aff" rid="a15"><sup>15</sup></xref></contrib><contrib contrib-type="author"><name><surname>Heizmann</surname><given-names>F.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Helbing</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a15"><sup>15</sup></xref></contrib><contrib contrib-type="author"><name><surname>Hickford</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a1 a15"><sup>1,15</sup></xref></contrib><contrib contrib-type="author"><name><surname>Hilk</surname><given-names>D.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Hillen</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Hillesheimer</surname><given-names>D.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Hinz</surname><given-names>D.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Höhn</surname><given-names>T.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Holzapfel</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a2"><sup>2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Holzmann</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a2"><sup>2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Houdy</surname><given-names>T.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Howe</surname><given-names>M. A.</given-names></name><xref ref-type="aff" rid="a13 a14"><sup>13,14</sup></xref></contrib><contrib contrib-type="author"><name><surname>Huber</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>James</surname><given-names>T. M.</given-names></name><xref ref-type="aff" rid="a2"><sup>2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Jansen</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kaboth</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a7"><sup>7</sup></xref></contrib><contrib contrib-type="author"><name><surname>Karl</surname><given-names>C.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kazachenko</surname><given-names>O.</given-names></name><xref ref-type="aff" rid="a21"><sup>21</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kellerer</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kernert</surname><given-names>N.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kippenbrock</surname><given-names>L.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kleesiek</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref><xref ref-type="author-notes" rid="n5"><sup>∥</sup></xref></contrib><contrib contrib-type="author"><name><surname>Klein</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a1 a6"><sup>1,6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Köhler</surname><given-names>C.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Köllenberger</surname><given-names>L.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kopmann</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Korzeczek</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kosmider</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kovalík</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a17"><sup>17</sup></xref></contrib><contrib contrib-type="author"><name><surname>Krasch</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kraus</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Krause</surname><given-names>H.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kuckert</surname><given-names>L.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref><xref ref-type="author-notes" rid="n6"><sup>¶</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kuffner</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Kunka</surname><given-names>N.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Lasserre</surname><given-names>T.</given-names></name><xref ref-type="aff" rid="a4 a3 a10"><sup>4,3,10</sup></xref></contrib><contrib contrib-type="author"><name><surname>Le</surname><given-names>T. L.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Lebeda</surname><given-names>O.</given-names></name><xref ref-type="aff" rid="a17"><sup>17</sup></xref></contrib><contrib contrib-type="author"><name><surname>Leber</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Lehnert</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a19"><sup>19</sup></xref></contrib><contrib contrib-type="author"><name><surname>Letnev</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a20"><sup>20</sup></xref></contrib><contrib contrib-type="author"><name><surname>Leven</surname><given-names>F.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Lichter</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Lobashev</surname><given-names>V. M.</given-names></name><xref ref-type="aff" rid="a21"><sup>21</sup></xref><xref ref-type="author-notes" rid="n1"><sup>,*</sup></xref></contrib><contrib contrib-type="author"><name><surname>Lokhov</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a8 a21"><sup>8,21</sup></xref></contrib><contrib contrib-type="author"><name><surname>Machatschek</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib 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contrib-type="author"><name><surname>Menshikov</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Mertens</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a10 a3 a19 a1"><sup>10,3,19,1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Minter</surname><given-names>L. I.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref><xref ref-type="author-notes" rid="n7"><sup>**</sup></xref></contrib><contrib contrib-type="author"><name><surname>Mirz</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Monreal</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a22"><sup>22</sup></xref></contrib><contrib contrib-type="author"><name><surname>Morales Guzmán</surname><given-names>P. I.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Müller</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Naumann</surname><given-names>U.</given-names></name><xref ref-type="aff" rid="a15"><sup>15</sup></xref></contrib><contrib contrib-type="author"><name><surname>Ndeke</surname><given-names>W.</given-names></name><xref ref-type="aff" rid="a25"><sup>25</sup></xref></contrib><contrib contrib-type="author"><name><surname>Neumann</surname><given-names>H.</given-names></name><xref ref-type="aff" rid="a2"><sup>2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Niemes</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Noe</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a2"><sup>2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Oblath</surname><given-names>N. S.</given-names></name><xref ref-type="aff" rid="a7"><sup>7</sup></xref></contrib><contrib contrib-type="author"><name><surname>Ortjohann</surname><given-names>H.-W.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Osipowicz</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a20"><sup>20</sup></xref></contrib><contrib contrib-type="author"><name><surname>Ostrick</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Otten</surname><given-names>E.</given-names></name><xref ref-type="aff" rid="a12"><sup>12</sup></xref><xref ref-type="author-notes" rid="n1"><sup>,*</sup></xref></contrib><contrib contrib-type="author"><name><surname>Parno</surname><given-names>D. S.</given-names></name><xref ref-type="aff" rid="a18 a16"><sup>18,16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Phillips</surname><given-names>D. G.</given-names><suffix>II</suffix></name><xref ref-type="aff" rid="a13 a14"><sup>13,14</sup></xref></contrib><contrib contrib-type="author"><name><surname>Plischke</surname><given-names>P.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Pollithy</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Poon</surname><given-names>A. W. P.</given-names></name><xref ref-type="aff" rid="a19"><sup>19</sup></xref></contrib><contrib contrib-type="author"><name><surname>Pouryamout</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a15"><sup>15</sup></xref></contrib><contrib contrib-type="author"><name><surname>Prall</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Priester</surname><given-names>F.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Röllig</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Röttele</surname><given-names>C.</given-names></name><xref ref-type="aff" rid="a1 a6 a2"><sup>1,6,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Ranitzsch</surname><given-names>P. C.-O.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Rest</surname><given-names>O.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Rinderspacher</surname><given-names>R.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Robertson</surname><given-names>R. G. H.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Rodenbeck</surname><given-names>C.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Rohr</surname><given-names>P.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Roll</surname><given-names>Ch.</given-names></name><xref ref-type="aff" rid="a25"><sup>25</sup></xref></contrib><contrib contrib-type="author"><name><surname>Rupp</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a1 a2 a6"><sup>1,2,6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Ryšavý</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a17"><sup>17</sup></xref></contrib><contrib contrib-type="author"><name><surname>Sack</surname><given-names>R.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Saenz</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a25"><sup>25</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schäfer</surname><given-names>P.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schimpf</surname><given-names>L.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schlösser</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schlösser</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schlüter</surname><given-names>L.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schön</surname><given-names>H.</given-names></name><xref ref-type="aff" rid="a2"><sup>2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schönung</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a11 a1 a2"><sup>11,1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schrank</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schulz</surname><given-names>B.</given-names></name><xref ref-type="aff" rid="a25"><sup>25</sup></xref></contrib><contrib contrib-type="author"><name><surname>Schwarz</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Seitz-Moskaliuk</surname><given-names>H.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Seller</surname><given-names>W.</given-names></name><xref ref-type="aff" rid="a20"><sup>20</sup></xref></contrib><contrib contrib-type="author"><name><surname>Sibille</surname><given-names>V.</given-names></name><xref ref-type="aff" rid="a7"><sup>7</sup></xref></contrib><contrib contrib-type="author"><name><surname>Siegmann</surname><given-names>D.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Skasyrskaya</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a21"><sup>21</sup></xref></contrib><contrib contrib-type="author"><name><surname>Slezák</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a10 a17"><sup>10,17</sup></xref></contrib><contrib contrib-type="author"><name><surname>Špalek</surname><given-names>A.</given-names></name><xref ref-type="aff" rid="a17"><sup>17</sup></xref></contrib><contrib contrib-type="author"><name><surname>Spanier</surname><given-names>F.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Steidl</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Steinbrink</surname><given-names>N.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Sturm</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Suesser</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a2"><sup>2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Sun</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Tcherniakhovski</surname><given-names>D.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Telle</surname><given-names>H. H.</given-names></name><xref ref-type="aff" rid="a23"><sup>23</sup></xref></contrib><contrib contrib-type="author"><name><surname>Thümmler</surname><given-names>T.</given-names></name><xref ref-type="aff" rid="a1 a8"><sup>1,8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Thorne</surname><given-names>L. A.</given-names></name><xref ref-type="aff" rid="a18"><sup>18</sup></xref></contrib><contrib contrib-type="author"><name><surname>Titov</surname><given-names>N.</given-names></name><xref ref-type="aff" rid="a21"><sup>21</sup></xref></contrib><contrib contrib-type="author"><name><surname>Tkachev</surname><given-names>I.</given-names></name><xref ref-type="aff" rid="a21"><sup>21</sup></xref></contrib><contrib contrib-type="author"><name><surname>Trost</surname><given-names>N.</given-names></name><xref ref-type="aff" rid="a1"><sup>1</sup></xref></contrib><contrib contrib-type="author"><name><surname>Urban</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a10 a3"><sup>10,3</sup></xref></contrib><contrib contrib-type="author"><name><surname>Vénos</surname><given-names>D.</given-names></name><xref ref-type="aff" rid="a17"><sup>17</sup></xref></contrib><contrib contrib-type="author"><name><surname>Valerius</surname><given-names>K.</given-names></name><xref ref-type="aff" rid="a1 a8"><sup>1,8</sup></xref></contrib><contrib contrib-type="author"><name><surname>VanDevender</surname><given-names>B. A.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Vianden</surname><given-names>R.</given-names></name><xref ref-type="aff" rid="a5"><sup>5</sup></xref></contrib><contrib contrib-type="author"><name><surname>Vizcaya Hernández</surname><given-names>A. P.</given-names></name><xref ref-type="aff" rid="a18"><sup>18</sup></xref></contrib><contrib contrib-type="author"><name><surname>Wall</surname><given-names>B. L.</given-names></name><xref ref-type="aff" rid="a16"><sup>16</sup></xref></contrib><contrib contrib-type="author"><name><surname>Wüstling</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><name><surname>Weber</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a9"><sup>9</sup></xref></contrib><contrib contrib-type="author"><contrib-id contrib-id-type="orcid">https://orcid.org/0000-0002-4083-9068</contrib-id><name><surname>Weinheimer</surname><given-names>C.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref><xref ref-type="author-notes" rid="n3"><sup>‡</sup></xref></contrib><contrib contrib-type="author"><name><surname>Weiss</surname><given-names>C.</given-names></name><xref ref-type="aff" rid="a24"><sup>24</sup></xref></contrib><contrib contrib-type="author"><name><surname>Welte</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Wendel</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="author"><name><surname>Wierman</surname><given-names>K. J.</given-names></name><xref ref-type="aff" rid="a13 a14"><sup>13,14</sup></xref></contrib><contrib contrib-type="author"><name><surname>Wilkerson</surname><given-names>J. F.</given-names></name><xref ref-type="aff" rid="a13 a14"><sup>13,14</sup></xref><xref ref-type="author-notes" rid="n8"><sup>††</sup></xref></contrib><contrib contrib-type="author"><name><surname>Wolf</surname><given-names>J.</given-names></name><xref ref-type="aff" rid="a6"><sup>6</sup></xref></contrib><contrib contrib-type="author"><name><surname>Xu</surname><given-names>W.</given-names></name><xref ref-type="aff" rid="a7"><sup>7</sup></xref></contrib><contrib contrib-type="author"><name><surname>Yen</surname><given-names>Y.-R.</given-names></name><xref ref-type="aff" rid="a18"><sup>18</sup></xref></contrib><contrib contrib-type="author"><name><surname>Zacher</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a8"><sup>8</sup></xref></contrib><contrib contrib-type="author"><name><surname>Zadorozhny</surname><given-names>S.</given-names></name><xref ref-type="aff" rid="a21"><sup>21</sup></xref></contrib><contrib contrib-type="author"><name><surname>Zbořil</surname><given-names>M.</given-names></name><xref ref-type="aff" rid="a8 a17"><sup>8,17</sup></xref></contrib><contrib contrib-type="author"><name><surname>Zeller</surname><given-names>G.</given-names></name><xref ref-type="aff" rid="a1 a2"><sup>1,2</sup></xref></contrib><contrib contrib-type="collaboration"><collab>(KATRIN Collaboration)</collab></contrib><aff id="a1"><label><sup>1</sup></label><institution>Institute for Nuclear Physics (IKP)</institution>, Karlsruhe Institute of Technology (KIT), Hermann-von-Helmholtz-Platz 1, 76344 Eggenstein-Leopoldshafen, Germany</aff><aff id="a2"><label><sup>2</sup></label><institution>Institute for Technical Physics (ITEP)</institution>, Karlsruhe Institute of Technology (KIT), Hermann-von-Helmholtz-Platz 1, 76344 Eggenstein-Leopoldshafen, Germany</aff><aff id="a3"><label><sup>3</sup></label><institution>Technische Universität München</institution>, James-Franck-Straße 1, 85748 Garching, Germany</aff><aff id="a4"><label><sup>4</sup></label>IRFU (DPhP &amp; APC), CEA, <institution>Université Paris-Saclay</institution>, 91191 Gif-sur-Yvette, France</aff><aff id="a5"><label><sup>5</sup></label>Helmholtz-Institut für Strahlen- und Kernphysik, <institution>Rheinische Friedrich-Wilhelms-Universität Bonn</institution>, Nussallee 14-16, 53115 Bonn, Germany</aff><aff id="a6"><label><sup>6</sup></label><institution>Institute of Experimental Particle Physics (ETP)</institution>, Karlsruhe Institute of Technology (KIT), Wolfgang-Gaede-Straße 1, 76131 Karlsruhe, Germany</aff><aff id="a7"><label><sup>7</sup></label>Laboratory for Nuclear Science, <institution>Massachusetts Institute of Technology</institution>, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, USA</aff><aff id="a8"><label><sup>8</sup></label>Institut für Kernphysik, <institution>Westfälische Wilhelms-Universität Münster</institution>, Wilhelm-Klemm-Straße 9, 48149 Münster, Germany</aff><aff id="a9"><label><sup>9</sup></label><institution>Institute for Data Processing and Electronics (IPE)</institution>, Karlsruhe Institute of Technology (KIT), Hermann-von-Helmholtz-Platz 1, 76344 Eggenstein-Leopoldshafen, Germany</aff><aff id="a10"><label><sup>10</sup></label><institution>Max-Planck-Institut für Physik</institution>, Föhringer Ring 6, 80805 München, Germany</aff><aff id="a11"><label><sup>11</sup></label><institution>Max-Planck-Institut für Kernphysik</institution>, Saupfercheckweg 1, 69117 Heidelberg, Germany</aff><aff id="a12"><label><sup>12</sup></label>Institut für Physik, <institution>Johannes-Gutenberg-Universität Mainz</institution>, 55099 Mainz, Germany</aff><aff id="a13"><label><sup>13</sup></label>Department of Physics and Astronomy, <institution>University of North Carolina</institution>, Chapel Hill, North Carolina 27599, USA</aff><aff id="a14"><label><sup>14</sup></label><institution>Triangle Universities Nuclear Laboratory</institution>, Durham, North Carolina 27708, USA</aff><aff id="a15"><label><sup>15</sup></label>Department of Physics, Faculty of Mathematics and Natural Sciences, <institution>University of Wuppertal</institution>, Gaußstraße 20, 42119 Wuppertal, Germany</aff><aff id="a16"><label><sup>16</sup></label>Center for Experimental Nuclear Physics and Astrophysics, and Department of Physics, <institution>University of Washington</institution>, Seattle, Washington 98195, USA</aff><aff id="a17"><label><sup>17</sup></label><institution>Nuclear Physics Institute of the CAS</institution>, v. v. i., CZ-250 68 Řež, Czech Republic</aff><aff id="a18"><label><sup>18</sup></label>Department of Physics, <institution>Carnegie Mellon University</institution>, Pittsburgh, Pennsylvania 15213, USA</aff><aff id="a19"><label><sup>19</sup></label><institution>Institute for Nuclear and Particle Astrophysics and Nuclear Science Division</institution>, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA</aff><aff id="a20"><label><sup>20</sup></label><institution>University of Applied Sciences (HFD) Fulda</institution>, Leipziger Straße 123, 36037 Fulda, Germany</aff><aff id="a21"><label><sup>21</sup></label><institution>Institute for Nuclear Research of Russian Academy of Sciences</institution>, 60th October Anniversary Prospect 7a, 117312 Moscow, Russia</aff><aff id="a22"><label><sup>22</sup></label>Department of Physics, <institution>Case Western Reserve University</institution>, Cleveland, Ohio 44106, USA</aff><aff id="a23"><label><sup>23</sup></label>Departamento de Química Física Aplicada, <institution>Universidad Autonoma de Madrid</institution>, Campus de Cantoblanco, 28049 Madrid, Spain</aff><aff id="a24"><label><sup>24</sup></label>Project, Process, and Quality Management (PPQ), <institution>Karlsruhe Institute of Technology (KIT)</institution>, Hermann-von-Helmholtz-Platz 1, 76344 Eggenstein-Leopoldshafen, Germany</aff><aff id="a25"><label><sup>25</sup></label>Institut für Physik, <institution>Humboldt-Universität zu Berlin</institution>, Newtonstraße 15, 12489 Berlin, Germany</aff></contrib-group><author-notes><fn id="n1"><label><sup>*</sup></label><p>Deceased.</p></fn><fn id="n2"><label><sup>†</sup></label><p>Corresponding author.</p><p><email>guido.drexlin@kit.edu</email></p></fn><fn id="n3"><label><sup>‡</sup></label><p>Corresponding author.</p><p><email>weinheimer@uni-muenster.de</email></p></fn><fn id="n4"><label><sup>§</sup></label><p>Formerly. K. Bokeloh (née Hugenberg)</p></fn><fn id="n5"><label><sup>∥</sup></label><p>Formerly. M. Kleesiek (né Haag)</p></fn><fn id="n6"><label><sup>¶</sup></label><p>Formerly. L. Kuckert (née Neumann)</p></fn><fn id="n7"><label><sup>**</sup></label><p>Formerly. L. I. Minter (née Bodine)</p></fn><fn id="n8"><label><sup>††</sup></label><p>Also at: Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA.</p></fn></author-notes><pub-date iso-8601-date="2019-11-25" date-type="pub" publication-format="electronic"><day>25</day><month>November</month><year>2019</year></pub-date><pub-date iso-8601-date="2019-11-29" date-type="pub" publication-format="print"><day>29</day><month>November</month><year>2019</year></pub-date><volume>123</volume><issue>22</issue><elocation-id>221802</elocation-id><pub-history><event><date iso-8601-date="2019-09-18" date-type="received"><day>18</day><month>September</month><year>2019</year></date></event></pub-history><permissions><copyright-statement>Published by the American Physical Society</copyright-statement><copyright-year>2019</copyright-year><copyright-holder>authors</copyright-holder><license license-type="creative-commons" xlink:href="https://creativecommons.org/licenses/by/4.0/"><license-p content-type="usage-statement">Published by the American Physical Society under the terms of the <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">Creative Commons Attribution 4.0 International</ext-link> license. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI. Funded by SCOAP<sup>3</sup>.</license-p></license></permissions><abstract><p>We report on the neutrino mass measurement result from the first four-week science run of the Karlsruhe Tritium Neutrino experiment KATRIN in spring 2019. Beta-decay electrons from a high-purity gaseous molecular tritium source are energy analyzed by a high-resolution MAC-E filter. A fit of the integrated electron spectrum over a narrow interval around the kinematic end point at 18.57 keV gives an effective neutrino mass square value of <inline-formula><mml:math display="inline"><mml:mo stretchy="false">(</mml:mo><mml:mo>-</mml:mo><mml:msubsup><mml:mn>1.0</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn>1.1</mml:mn></mml:mrow><mml:mrow><mml:mo>+</mml:mo><mml:mn>0.9</mml:mn></mml:mrow></mml:msubsup><mml:mo stretchy="false">)</mml:mo><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:msup><mml:mrow><mml:mi>eV</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. From this, we derive an upper limit of 1.1 eV (90% confidence level) on the absolute mass scale of neutrinos. This value coincides with the KATRIN sensitivity. It improves upon previous mass limits from kinematic measurements by almost a factor of 2 and provides model-independent input to cosmological studies of structure formation.</p></abstract><funding-group><award-group award-type="unspecified"><funding-source country="DE"><institution-wrap><institution>Helmholtz Association</institution><institution-id institution-id-type="doi" vocab="open-funder-registry" vocab-identifier="10.13039/open-funder-registry">10.13039/501100009318</institution-id></institution-wrap></funding-source><award-id>VH-NG-1055</award-id></award-group><award-group award-type="grant"><funding-source country="DE"><institution-wrap><institution>Bundesministerium für Bildung und Forschung</institution><institution-id institution-id-type="doi" vocab="open-funder-registry" vocab-identifier="10.13039/open-funder-registry">10.13039/501100002347</institution-id></institution-wrap></funding-source><award-id>5A17PDA</award-id><award-id>05A17PM3</award-id><award-id>05A17PX3</award-id><award-id>05A17VK2</award-id><award-id>05A17WO3</award-id></award-group><award-group award-type="unspecified"><funding-source country="DE"><institution-wrap><institution>Max-Planck-Gesellschaft</institution><institution-id institution-id-type="doi" vocab="open-funder-registry" vocab-identifier="10.13039/open-funder-registry">10.13039/501100004189</institution-id></institution-wrap></funding-source></award-group><award-group award-type="grant"><funding-source country="DE"><institution-wrap><institution>Deutsche Forschungsgemeinschaft</institution><institution-id institution-id-type="doi" vocab="open-funder-registry" vocab-identifier="10.13039/open-funder-registry">10.13039/501100001659</institution-id></institution-wrap></funding-source><award-id>GRK 1694</award-id><award-id>GRK 2149</award-id><award-id>GSC 1085—KSETA</award-id></award-group><award-group award-type="grant"><funding-source country="CZ"><institution-wrap><institution>Ministerstvo Školství, Mládeže a T?lovýchovy</institution><institution-id institution-id-type="doi" vocab="open-funder-registry" vocab-identifier="10.13039/open-funder-registry">10.13039/501100001823</institution-id></institution-wrap></funding-source><award-id>CANAM-LM2011019</award-id><award-id>LTT19005</award-id></award-group><award-group award-type="grant"><funding-source country="US"><institution-wrap><institution>U.S. Department of Energy</institution><institution-id institution-id-type="doi" vocab="open-funder-registry" vocab-identifier="10.13039/open-funder-registry">10.13039/100000015</institution-id></institution-wrap></funding-source><award-id>DE-FG02-97ER41020</award-id><award-id>DE-FG02-94ER40818</award-id><award-id>DE-SC0004036</award-id><award-id>DE-FG02-97ER41033</award-id><award-id>DE-FG02-97ER41041</award-id><award-id>DE-AC02-05CH11231</award-id><award-id>DE-SC0011091</award-id><award-id>DE-SC0019304</award-id></award-group><award-group award-type="unspecified"><funding-source country=""><institution-wrap><institution>National Energy Research Scientific Computing Center</institution></institution-wrap></funding-source></award-group></funding-group><counts><page-count count="10"/></counts><custom-meta-group><custom-meta><meta-name>marker</meta-name><meta-value>PHYSICS</meta-value></custom-meta><custom-meta><meta-name>marker</meta-name><meta-value>L_SUGG</meta-value></custom-meta></custom-meta-group></article-meta></front><body><sec id="s1"><title specific-use="run-in">Introduction.—</title><p>The observation of flavor oscillations of atmospheric and solar neutrinos <xref ref-type="bibr" rid="c1 c2">[1,2]</xref> as well as oscillation studies at reactors and accelerators unequivocally prove neutrinos to possess nonzero rest masses (e.g., <xref ref-type="bibr" rid="c3">[3]</xref>), contradicting the standard model (SM) expectation of them being massless. The absolute values <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:math></inline-formula> of the neutrino mass states <inline-formula><mml:math display="inline"><mml:msub><mml:mi>ν</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mi>i</mml:mi><mml:mo>=</mml:mo><mml:mn>1</mml:mn></mml:math></inline-formula>, 2, 3), which cannot be probed by oscillations, are of fundamental importance in cosmological studies <xref ref-type="bibr" rid="c4 c5 c6">[4–6]</xref> and for particle physics models beyond the SM <xref ref-type="bibr" rid="c7">[7]</xref>.</p><p>Because of the unique role of primordial neutrinos in the formation of large-scale structures in the universe, observations of matter clustering in different epochs of the universe allow one to probe the neutrino mass sum <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">Σ</mml:mi></mml:mrow><mml:mrow><mml:mi>i</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mrow><mml:mi>m</mml:mi></mml:mrow><mml:mrow><mml:mi>i</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>. The current upper limits depend on the selection of data sets included in the analyses and are valid only within the <inline-formula><mml:math display="inline"><mml:mi mathvariant="normal">Λ</mml:mi><mml:mi>CDM</mml:mi></mml:math></inline-formula> concordance model <xref ref-type="bibr" rid="c6 c8">[6,8]</xref>. Another model-dependent method is provided by the search for neutrinoless double beta decay <inline-formula><mml:math display="inline"><mml:mn>0</mml:mn><mml:mi>ν</mml:mi><mml:mi>β</mml:mi><mml:mi>β</mml:mi></mml:math></inline-formula>, a process forbidden in the SM due to lepton number violation. It gives access to the effective Majorana neutrino mass (e.g., <xref ref-type="bibr" rid="c9 c10">[9,10]</xref>).</p><p>A model-independent, direct method for probing the neutrino mass scale in the laboratory is provided by kinematic studies of weak-interaction processes such as <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> decay of tritium (<inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi mathvariant="normal">H</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula>) and electron capture on holmium (<inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Ho</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>163</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula>) <xref ref-type="bibr" rid="c11 c12 c13 c14 c15">[11–15]</xref>. These investigations yield an incoherent sum of spectra, containing the squares of the neutrino eigenmasses <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>i</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula> as parameters. Each spectral component is weighted by the absolute square of the corresponding electron-flavor matrix element <inline-formula><mml:math display="inline"><mml:mo stretchy="false">|</mml:mo><mml:msub><mml:mi>U</mml:mi><mml:mrow><mml:mi mathvariant="normal">e</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:msub><mml:msup><mml:mo stretchy="false">|</mml:mo><mml:mn>2</mml:mn></mml:msup></mml:math></inline-formula>. In the quasidegenerate regime <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>&gt;</mml:mo><mml:mn>0.2</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula>, the eigenmasses are the same to better than 3%. The mass measured in <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> decay or electron capture, often called “<inline-formula><mml:math display="inline"><mml:mi>m</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:msub><mml:mi>ν</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula>,” is the neutrino mass <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub><mml:mo>≈</mml:mo><mml:msub><mml:mi>m</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:math></inline-formula> in this regime.</p><p>Because of its low end point energy (<inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub><mml:mo>=</mml:mo><mml:mn>18.57</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>keV</mml:mi></mml:math></inline-formula>) and favorable half-life (<inline-formula><mml:math display="inline"><mml:msub><mml:mi>t</mml:mi><mml:mrow><mml:mn>1</mml:mn><mml:mo stretchy="false">/</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:mn>12.32</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>yr</mml:mi></mml:math></inline-formula>), the decay of tritium <inline-formula><mml:math display="inline"><mml:mrow><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi mathvariant="normal">H</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow><mml:mo stretchy="false">→</mml:mo><mml:mrow><mml:msup><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>He</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:mrow><mml:mo>+</mml:mo><mml:msup><mml:mrow><mml:mi>e</mml:mi></mml:mrow><mml:mrow><mml:mo>-</mml:mo></mml:mrow></mml:msup><mml:mo>+</mml:mo><mml:msub><mml:mrow><mml:mover accent="true"><mml:mrow><mml:mi>ν</mml:mi></mml:mrow><mml:mrow><mml:mo stretchy="false">¯</mml:mo></mml:mrow></mml:mover></mml:mrow><mml:mrow><mml:mi>e</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> has been investigated by a large number of experiments looking for the small, characteristic shape distortion of the <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> spectrum close to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> due to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub></mml:math></inline-formula> <xref ref-type="bibr" rid="c11 c12">[11,12]</xref>. Experimental advances over many decades have steadily increased the sensitivity to the present upper limit of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub><mml:mo>&lt;</mml:mo><mml:mn>2</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula> (95% confidence level, C.L.) <xref ref-type="bibr" rid="c16">[16]</xref>. In this Letter, we report on the first neutrino mass result from the Karlsruhe Tritium Neutrino experiment KATRIN <xref ref-type="bibr" rid="c17 c18 c19 c20">[17–20]</xref>, which is targeted to advance the sensitivity on <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub></mml:math></inline-formula> by 1 order of magnitude down to 0.2 eV (90% C.L.) after five years.</p></sec><sec id="s2"><title specific-use="run-in">Experimental setup.—</title><p>KATRIN combines a windowless gaseous molecular tritium source (WGTS), pioneered by the Los Alamos experiment <xref ref-type="bibr" rid="c21">[21]</xref>, with a spectrometer based on the principle of magnetic adiabatic collimation with electrostatic filtering (MAC-E-filter) <xref ref-type="bibr" rid="c22 c23">[22,23]</xref>, developed at Mainz and Troitsk <xref ref-type="bibr" rid="c24 c25">[24,25]</xref>. These techniques allow the investigation of the end point region of tritium <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> decay with very high energy resolution, large statistics, and small systematics. KATRIN has been designed and built to refine this direct kinematic method to its ultimate precision level. To improve the sensitivity on <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub></mml:math></inline-formula> by 1 order of magnitude calls for an increase in statistics and a reduction of systematic uncertainties by 2 orders of magnitude, as the observable in kinematic studies is the neutrino mass square, <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula>.</p><p>Figure <xref ref-type="fig" rid="f1">1</xref> gives an overview of the 70 m long experimental setup located at the Karlsruhe Institute of Technology. The source-related components in contact with tritium, the rear section (RS) (a), the WGTS cryostat (b), as well as the differential (DPS) and cryogenic (CPS) pumping sections (c) are integrated into the extensive infrastructure of Tritium Laboratory Karlsruhe to enable a closed cycle of tritium <xref ref-type="bibr" rid="c26">[26]</xref>. High-purity tritium gas from a pressure-controlled buffer vessel is continuously injected at 30 K into the WGTS at the midpoint of its 90 mm diameter, 10 m long stainless steel beam tube. The gas then diffuses to both ends where it is pumped out by a series of turbomolecular pumps (TMPs) in the DPS, yielding the nominal column density <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>ρ</mml:mi><mml:msub><mml:mrow><mml:mi>d</mml:mi></mml:mrow><mml:mrow><mml:mi>nom</mml:mi></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:mn>5</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mn>17</mml:mn></mml:mrow></mml:msup><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>molecules</mml:mi><mml:mtext> </mml:mtext><mml:msup><mml:mrow><mml:mi>cm</mml:mi></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. In combination with the CPS, housing a large-capacity cryotrap operated at around 3 K, the flow rate of tritium into the following spectrometer and detector section [Figs. <xref ref-type="fig" rid="f1">1(d)–1(f)</xref>] downstream is negligible, well below the 14 orders of magnitude of flow reduction required to eliminate source-related background by neutral tritium gas <xref ref-type="bibr" rid="c17">[17]</xref>.</p><fig id="f1"><object-id>1</object-id><object-id pub-id-type="doi">10.1103/PhysRevLett.123.221802.f1</object-id><label>FIG. 1.</label><caption><p>The major components of the KATRIN beam line consist of (a) the rear section for diagnostics, (b) the windowless gaseous tritium source WGTS, c) the pumping section with the DPS and CPS cryostats, and a tandem setup of two MAC-E-filters: (d) the smaller prespectrometer and (e) the larger main spectrometer with its surrounding air coil system. This system transmits only the highest-energy <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> decay electrons onto (f) the solid-state detector where they are counted.</p></caption><graphic xlink:href="e221802_1.eps"/></fig><p>The source magnetic field (section b) in Fig. <xref ref-type="fig" rid="f1">1</xref>, <inline-formula><mml:math display="inline"><mml:msub><mml:mi>B</mml:mi><mml:mrow><mml:mi>WGTS</mml:mi></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:mn>2.52</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mrow><mml:mi mathvariant="normal">T</mml:mi></mml:mrow></mml:math></inline-formula>) as well as other superconducting solenoids [section (c) in Fig. <xref ref-type="fig" rid="f1">1</xref>] <xref ref-type="bibr" rid="c27">[27]</xref> adiabatically guide primary <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay electrons, secondary electrons, and ions to the spectrometers. A series of blocking and dipole electrodes eliminates ions by an <inline-formula><mml:math display="inline"><mml:mrow><mml:mover accent="true"><mml:mrow><mml:mi>E</mml:mi></mml:mrow><mml:mrow><mml:mo stretchy="false">→</mml:mo></mml:mrow></mml:mover><mml:mo>×</mml:mo><mml:mover accent="true"><mml:mrow><mml:mi>B</mml:mi></mml:mrow><mml:mrow><mml:mo stretchy="false">→</mml:mo></mml:mrow></mml:mover></mml:mrow></mml:math></inline-formula> drift to the beam tube, so that they cannot generate background in the spectrometer section <xref ref-type="bibr" rid="c19">[19]</xref>.</p><p>High-precision electron spectroscopy is achieved by the MAC-E-filter technique, where electrons of charge <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> are guided by the magnetic field, collimated by its gradient and filtered by an electrostatic barrier, the retarding potential energy <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula>. The resulting high-pass filter transmits only electrons with enough energy to overcome the barrier <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula> and allows the scanning of the tritium <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay spectrum in an integral mode.</p><p>The tandem configuration of MAC-E-filters performs a two-step filter process: first, the smaller prespectrometer is operated at fixed high voltage (HV) of <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo><mml:mn>10.4</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>kV</mml:mi></mml:math></inline-formula> in this work to act as a prefilter to reject electrons that carry no information on <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub></mml:math></inline-formula>. In a second step, a variable <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula> is applied to the main spectrometer for precision filtering of <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay electrons close to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula>. Its huge size guarantees fully adiabatic motion to the central “analyzing plane,” where the minimum magnetic field <inline-formula><mml:math display="inline"><mml:msub><mml:mi>B</mml:mi><mml:mi>min</mml:mi></mml:msub></mml:math></inline-formula> and the maximum retarding energy <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula> coincide for the filtering process to occur. Elevating the two spectrometers to a negative HV forms a strong Penning trap which can give rise to background <xref ref-type="bibr" rid="c28 c29">[28,29]</xref>. This is avoided by operating both at an ultrahigh vacuum (UHV) regime of <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mn>11</mml:mn></mml:mrow></mml:msup><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>mbar</mml:mi></mml:mrow></mml:math></inline-formula> using nonevaporable getter (NEG) pumps and TMPs <xref ref-type="bibr" rid="c30">[30]</xref>.</p><p>A defining property of a MAC-E-filter is <inline-formula><mml:math display="inline"><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>E</mml:mi><mml:mo stretchy="false">/</mml:mo><mml:mi>E</mml:mi></mml:math></inline-formula>, the filter width at energy <inline-formula><mml:math display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula>, which is given by the ratio <inline-formula><mml:math display="inline"><mml:msub><mml:mi>B</mml:mi><mml:mi>min</mml:mi></mml:msub><mml:mo stretchy="false">/</mml:mo><mml:msub><mml:mi>B</mml:mi><mml:mi>max</mml:mi></mml:msub></mml:math></inline-formula> of the minimum to maximum magnetic field in nonrelativistic approximation. The present ratio (<inline-formula><mml:math display="inline"><mml:mrow><mml:mn>0.63</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>mT</mml:mi><mml:mo>/</mml:mo><mml:mn>4.24</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi mathvariant="normal">T</mml:mi></mml:mrow></mml:math></inline-formula>) is equivalent to <inline-formula><mml:math display="inline"><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>E</mml:mi><mml:mo>=</mml:mo><mml:mn>2.8</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula> at <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula>. This value constrains the size <inline-formula><mml:math display="inline"><mml:msub><mml:mi>V</mml:mi><mml:mi>ft</mml:mi></mml:msub></mml:math></inline-formula> of the flux tube around <inline-formula><mml:math display="inline"><mml:msub><mml:mi>B</mml:mi><mml:mi>min</mml:mi></mml:msub></mml:math></inline-formula> and, consequently, the overall background rate, which is proportional to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>V</mml:mi><mml:mi>ft</mml:mi></mml:msub></mml:math></inline-formula> to the first order. A large air coil system of 12.6 m diameter <xref ref-type="bibr" rid="c31">[31]</xref> is used to adjust <inline-formula><mml:math display="inline"><mml:msub><mml:mi>B</mml:mi><mml:mi>min</mml:mi></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:msub><mml:mi>V</mml:mi><mml:mi>ft</mml:mi></mml:msub></mml:math></inline-formula>. After the potential of the spectrometer vessel is elevated, an offset of up to <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo><mml:mn>200</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mrow><mml:mi mathvariant="normal">V</mml:mi></mml:mrow></mml:math></inline-formula> can be applied to the wire electrode system mounted on the inner surface of the vessel to define <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula>.</p><p>Electrons transmitted through the spectrometers are finally counted in a radially and azimuthally segmented monolithic silicon detector array with 148 pixels <xref ref-type="bibr" rid="c32">[32]</xref> as a function of <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula>. To optimize the signal-to-background ratio, transmitted electrons are postaccelerated by a potential of <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>+</mml:mo><mml:mn>10</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>kV</mml:mi></mml:mrow></mml:math></inline-formula> before they impinge on the detector.</p></sec><sec id="s3"><title specific-use="run-in">Commissioning measurements.—</title><p>Over the past years, we have commissioned the entire setup by a series of dedicated long-term measurements <xref ref-type="bibr" rid="c19 c26 c27 c33">[19,26,27,33]</xref> which have demonstrated that all specifications <xref ref-type="bibr" rid="c18">[18]</xref> are met, or even surpassed by up to 1 order of magnitude, except for the background rate <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula>.</p><p>A major benchmark is to operate the source at <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:msub><mml:mi>d</mml:mi><mml:mi>nom</mml:mi></mml:msub></mml:math></inline-formula> at a stability level of <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mn>3</mml:mn></mml:mrow></mml:msup><mml:mo>/</mml:mo><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> so that variations of the column density <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi></mml:math></inline-formula> can be neglected. This calls for a stable gas injection rate via capillaries <xref ref-type="bibr" rid="c26">[26]</xref> and a constant beam-tube temperature. For the latter, a stability level of better than <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mn>3</mml:mn></mml:mrow></mml:msup><mml:mo>/</mml:mo><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> has been achieved by a two-phase beam-tube cooling system at 30 (100) K using neon (argon) as a cooling fluid <xref ref-type="bibr" rid="c34">[34]</xref>. In mid-2018, measurements at 1% DT concentration within a 99% <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">D</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> carrier gas at <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:msub><mml:mi>d</mml:mi><mml:mi>nom</mml:mi></mml:msub></mml:math></inline-formula> have verified the required level of source stability <xref ref-type="bibr" rid="c35">[35]</xref>. This “first tritium” campaign has allowed us to collect the first integral electron spectra which agree well with the model expectation.</p><p>In this spectral comparison, the response function <inline-formula><mml:math display="inline"><mml:mi>f</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> <xref ref-type="bibr" rid="c20">[20]</xref> plays a fundamental role [see Eq. <xref ref-type="disp-formula" rid="d1">(1)</xref>], as it converts the theoretical <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> spectrum into the experimental spectrum. It describes the probability of transmission of an electron with initial energy <inline-formula><mml:math display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula> as a function of its surplus energy <inline-formula><mml:math display="inline"><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula>. For an ensemble, it depends on the angular spread of electrons and the amount of neutral gas they pass in the source, where they can undergo inelastic scattering processes with a total cross section <inline-formula><mml:math display="inline"><mml:mi>σ</mml:mi></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mrow><mml:mn>3.64</mml:mn><mml:mo>×</mml:mo><mml:mrow><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mn>18</mml:mn></mml:mrow></mml:msup><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:msup><mml:mrow><mml:mi>cm</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:mrow></mml:math></inline-formula> at 18.57 keV, adopted from <xref ref-type="bibr" rid="c36">[36]</xref>).</p><p>We measure <inline-formula><mml:math display="inline"><mml:mi>f</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> using monoenergetic electrons with a small angular spread produced in a dedicated photoelectron source (<inline-formula><mml:math display="inline"><mml:mi>e</mml:mi></mml:math></inline-formula> gun) <xref ref-type="bibr" rid="c37">[37]</xref> located at the RS. These electrons span a 50 eV wide range of surplus energies <inline-formula><mml:math display="inline"><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula> and pass through the integral column density <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi></mml:math></inline-formula> of the source. This allows us to measure the characteristics of single (<inline-formula><mml:math display="inline"><mml:mi>s</mml:mi><mml:mo>=</mml:mo><mml:mn>1</mml:mn></mml:math></inline-formula>) and multiple (<inline-formula><mml:math display="inline"><mml:mi>s</mml:mi><mml:mo>=</mml:mo><mml:mn>2</mml:mn><mml:mo>,</mml:mo><mml:mn>3</mml:mn><mml:mo>,</mml:mo><mml:mo>…</mml:mo></mml:math></inline-formula>) inelastic scattering in <inline-formula><mml:math display="inline"><mml:msub><mml:mi>T</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math></inline-formula>. In Fig. <xref ref-type="fig" rid="f2">2</xref> (top), we display the measured response <inline-formula><mml:math display="inline"><mml:mi>f</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> for a narrow-angle photoelectron source as well as the calculated response <inline-formula><mml:math display="inline"><mml:msub><mml:mi>f</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> for isotropically emitted <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay electrons for the normal integrating MAC-E mode for <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi><mml:mo>≈</mml:mo><mml:mi>ρ</mml:mi><mml:msub><mml:mi>d</mml:mi><mml:mi>nom</mml:mi></mml:msub></mml:math></inline-formula>. The sharp rise with the filter width <inline-formula><mml:math display="inline"><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>E</mml:mi></mml:math></inline-formula> to a plateau extending up to 11 eV results from “no loss” (energy loss <inline-formula><mml:math display="inline"><mml:mi>δ</mml:mi><mml:mi>E</mml:mi><mml:mo>=</mml:mo><mml:mn>0</mml:mn></mml:math></inline-formula>) <inline-formula><mml:math display="inline"><mml:mi>e</mml:mi></mml:math></inline-formula>-gun electrons, which leave the source without scattering (<inline-formula><mml:math display="inline"><mml:mi>s</mml:mi><mml:mo>=</mml:mo><mml:mn>0</mml:mn></mml:math></inline-formula>) with a probability <inline-formula><mml:math display="inline"><mml:mi>exp</mml:mi><mml:mrow><mml:mo stretchy="false">(</mml:mo><mml:mo>-</mml:mo><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi><mml:mo>·</mml:mo><mml:mi>σ</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula>. At larger <inline-formula><mml:math display="inline"><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math display="inline"><mml:mi>s</mml:mi></mml:math></inline-formula>-fold scattering (<inline-formula><mml:math display="inline"><mml:mi>s</mml:mi><mml:mo>=</mml:mo><mml:mn>1</mml:mn></mml:math></inline-formula>, 2, 3) is visible. In Fig. <xref ref-type="fig" rid="f2">2</xref> (bottom), the differential data from the MAC-E-TOF mode <xref ref-type="bibr" rid="c38">[38]</xref> are shown, where the electron time of flight (TOF) is recorded. This allows us to even better assess the <inline-formula><mml:math display="inline"><mml:mi>s</mml:mi></mml:math></inline-formula>-fold inelastic scattering and to obtain the energy-loss function of electrons <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>ϵ</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>δ</mml:mi><mml:mi>E</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula> by a deconvolution with the no loss peak at <inline-formula><mml:math display="inline"><mml:mi>δ</mml:mi><mml:mi>E</mml:mi><mml:mo>=</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo>=</mml:mo><mml:mn>0</mml:mn></mml:math></inline-formula>.</p><fig id="f2"><object-id>2</object-id><object-id pub-id-type="doi">10.1103/PhysRevLett.123.221802.f2</object-id><label>FIG. 2.</label><caption><p>(top) Measured and calculated response functions <inline-formula><mml:math display="inline"><mml:mi>f</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> for electron surplus energies <inline-formula><mml:math display="inline"><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula> at different <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi></mml:math></inline-formula> values of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>T</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math></inline-formula>. Measured <inline-formula><mml:math display="inline"><mml:mi>f</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> for a narrow-angle photoelectron source close to <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:msub><mml:mi>d</mml:mi><mml:mi>nom</mml:mi></mml:msub></mml:math></inline-formula> and fit (cyan line); and calculated <inline-formula><mml:math display="inline"><mml:msub><mml:mi>f</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> for isotropically emitted <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> decay electrons up to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>θ</mml:mi><mml:mi>max</mml:mi></mml:msub></mml:math></inline-formula> at <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:msub><mml:mi>d</mml:mi><mml:mi>exp</mml:mi></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1.11</mml:mn><mml:mo>×</mml:mo><mml:mrow><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mn>17</mml:mn></mml:mrow></mml:msup><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mrow><mml:msup><mml:mrow><mml:mi>cm</mml:mi></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:mrow></mml:mrow></mml:math></inline-formula>), the set point of our scans (red line), and in the limit of vanishing <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi><mml:mo>=</mml:mo><mml:mn>0</mml:mn></mml:math></inline-formula> (grey, dashed-dotted line). (bottom) Differential distributions of energy losses <inline-formula><mml:math display="inline"><mml:mi>δ</mml:mi><mml:mi>E</mml:mi></mml:math></inline-formula> from the MAC-E-TOF mode after a selection <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>35</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>μ</mml:mi><mml:mi mathvariant="normal">s</mml:mi><mml:mo>≤</mml:mo><mml:mi>TOF</mml:mi><mml:mo>≤</mml:mo><mml:mn>50</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>μ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> at <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi><mml:mo>≈</mml:mo><mml:mi>ρ</mml:mi><mml:msub><mml:mi>d</mml:mi><mml:mi>nom</mml:mi></mml:msub></mml:math></inline-formula> and fit (cyan line). The “no loss” peak at <inline-formula><mml:math display="inline"><mml:mi>δ</mml:mi><mml:mi>E</mml:mi><mml:mo>=</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo>=</mml:mo><mml:mn>0</mml:mn></mml:math></inline-formula> is followed by peaks with <inline-formula><mml:math display="inline"><mml:mi>s</mml:mi><mml:mo>=</mml:mo><mml:mn>2</mml:mn></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mi>s</mml:mi><mml:mo>=</mml:mo><mml:mn>3</mml:mn></mml:math></inline-formula>) scattering at twice (triple) the <inline-formula><mml:math display="inline"><mml:mi>δ</mml:mi><mml:mi>E</mml:mi></mml:math></inline-formula> value of <inline-formula><mml:math display="inline"><mml:mi>s</mml:mi><mml:mo>=</mml:mo><mml:mn>1</mml:mn></mml:math></inline-formula>. The energy loss function <inline-formula><mml:math display="inline"><mml:mi>ϵ</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>δ</mml:mi><mml:mi>E</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> for <inline-formula><mml:math display="inline"><mml:mi>s</mml:mi><mml:mo>=</mml:mo><mml:mn>1</mml:mn></mml:math></inline-formula> is obtained by deconvolution (orange line).</p></caption><graphic xlink:href="e221802_2.eps"/></fig><p>As the background rate <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula> exceeds its design goal of 0.01 counts per second (cps), we have studied the nature and origin of background processes so as to implement mitigation measures. Up to now, source-related backgrounds have not been observed, so that spectrometer-related processes <xref ref-type="bibr" rid="c39">[39]</xref> dominate <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula> apart from a small detector-related contribution <xref ref-type="bibr" rid="c32">[32]</xref>. Electrons generated at the spectrometer surface by cosmic muons and environmental gamma rays are inhibited from entering the inner flux tube by magnetic and electric barriers <xref ref-type="bibr" rid="c40 c41">[40,41]</xref>. Thus, <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>bg</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> originates from excited or unstable neutral atoms which can propagate freely in the UHV environment. Accordingly, <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula> is observed to have an almost constant rate per unit volume in the flux tube.</p><p>Detailed investigations of the background behavior <xref ref-type="bibr" rid="c39 c42">[39,42]</xref> revealed that a significant part of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula> is due to Rydberg atoms sputtered off the inner spectrometer surfaces by <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Pb</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>206</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula>-recoil ions following <inline-formula><mml:math display="inline"><mml:mi>α</mml:mi></mml:math></inline-formula> decays of <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Po</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>210</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula>. These processes follow the decay chain of the long-lived <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Rn</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>222</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula> progeny <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Pb</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>210</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula>, which was surface-implanted from ambient air (activity <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>≈</mml:mo><mml:mn>1</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>Bq</mml:mi><mml:mo>/</mml:mo><mml:msup><mml:mrow><mml:mi mathvariant="normal">m</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>) during the construction phase. A small fraction of these Rydberg states is ionized by black-body radiation when propagating over the magnetic flux tube. The resulting sub-eV scale electrons are accelerated to <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula> by the MAC-E-filter and form a Poisson component to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula>.</p><p>The other part of background events stems from <inline-formula><mml:math display="inline"><mml:mi>α</mml:mi></mml:math></inline-formula> decays of single <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Rn</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>219</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula> atoms (<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>t</mml:mi></mml:mrow><mml:mrow><mml:mn>1</mml:mn><mml:mo stretchy="false">/</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:mn>3.96</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula>) emanating from the NEG pumps located in two of the three pump ports of the main spectrometer which release a large number of electrons up to the keV scale in the flux tube, where they are stored due to its magnetic bottle characteristics. By scattering off residual gas, the stored electrons subsequently produce secondary background electrons. This process continues until the stored electron is cooled off to an energy of a few eV when it can escape and also contribute itself to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula> at <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula>. Owing to its origin from a small number of <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Rn</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>219</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula> decays, this background results in extended time periods where the background level is enhanced yielding a small non-Poissonian component <xref ref-type="bibr" rid="c43">[43]</xref>. Liquid-nitrogen cooled copper baffles at the inlet of the NEG pumps act as a countermeasure <xref ref-type="bibr" rid="c44">[44]</xref>. The coverage of the inner surface of the main spectrometer with a monolayer of <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">H</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub><mml:mi mathvariant="normal">O</mml:mi></mml:mrow></mml:math></inline-formula>, originating from an imperfect bake out of the prespectrometer, has led to the formation of a thin layer of <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">H</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub><mml:mi mathvariant="normal">O</mml:mi></mml:mrow></mml:math></inline-formula> covering the baffle surface. Therefore, the retention of <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Rn</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>219</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula> in this work is hampered such that <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula> retains a small non-Poissonian component.</p></sec><sec id="s4"><title specific-use="run-in">Measurements of the tritium <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> spectrum.—</title><p>In the following, we report on our first high-purity tritium campaign from April 10 to May 13, 2019 which demonstrates the functionality of all system components and of the extensive tritium infrastructure at large source activity (<inline-formula><mml:math display="inline"><mml:mn>2.45</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mn>10</mml:mn></mml:msup><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>Bq</mml:mi></mml:math></inline-formula>) and tritium throughput (<inline-formula><mml:math display="inline"><mml:mrow><mml:mn>4.9</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi mathvariant="normal">g</mml:mi><mml:mo>/</mml:mo><mml:mi>day</mml:mi></mml:mrow></mml:math></inline-formula>). As a result of radiochemical reactions of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>T</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math></inline-formula> with the previously unexposed inner metal surface of the injection capillary, we observe drifts in the source column density. To limit these drifts to a level of <inline-formula><mml:math display="inline"><mml:mo>±</mml:mo><mml:mn>2</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> over our campaign, we keep the column density at an average value of <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>ρ</mml:mi><mml:msub><mml:mrow><mml:mi>d</mml:mi></mml:mrow><mml:mrow><mml:mi>exp</mml:mi></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:mn>1.11</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mn>17</mml:mn></mml:mrow></mml:msup><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>molecules</mml:mi><mml:mtext> </mml:mtext><mml:msup><mml:mrow><mml:mi>cm</mml:mi></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, which is about a factor of 5 smaller than <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:msub><mml:mi>d</mml:mi><mml:mi>nom</mml:mi></mml:msub></mml:math></inline-formula>.</p><p> At this setting, the smaller value of <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:msub><mml:mi>d</mml:mi><mml:mi>exp</mml:mi></mml:msub><mml:mo>·</mml:mo><mml:mi>σ</mml:mi></mml:math></inline-formula> (0.404) reduces the amount of inelastic scattering of electrons off neutral gas, see Fig. <xref ref-type="fig" rid="f2">2</xref>. The relative fractions of the six hydrogen isotopologues injected into the source are continuously monitored by laser-Raman spectroscopy with <inline-formula><mml:math display="inline"><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn>3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> precision <xref ref-type="bibr" rid="c45">[45]</xref>. The average isotopic tritium purity <inline-formula><mml:math display="inline"><mml:msub><mml:mi>ϵ</mml:mi><mml:mi>T</mml:mi></mml:msub></mml:math></inline-formula> (0.976) of our analyzed data sample is derived from the composition of the tritiated species <inline-formula><mml:math display="inline"><mml:msub><mml:mi>T</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math></inline-formula> (0.953), HT (0.035), and DT (0.011), with inactive species (<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">D</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, HD, and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">H</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>) being present only in trace amounts.</p><p>Because of the large number of <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> decay s and ionization processes, a cold magnetized plasma of electrons (meV to keV scale) and ions (meV scale) is formed which interacts with the neutral gas. The strong solenoidal field <inline-formula><mml:math display="inline"><mml:msub><mml:mrow><mml:mi mathvariant="normal">B</mml:mi></mml:mrow><mml:mrow><mml:mi>WGTS</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula> and the resulting large longitudinal conductance of the plasma allow the coupling of its potential to the surface of the rear wall (RW) located at the RS and, thus, to control the starting energies of <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay electrons over the volume <xref ref-type="bibr" rid="c46">[46]</xref>. Biasing the gold-plated RW disk with small areal variation of the work function to <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo><mml:mn>0.15</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mrow><mml:mi mathvariant="normal">V</mml:mi></mml:mrow></mml:math></inline-formula> relative to the grounded beam tube gives a very good radial homogeneity of the source potential. This is verified during initial tritium scans with fits of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> over detector pixel rings, which do not show a significant radial variation.</p><p>Additional information on plasma effects is provided by comparing the line shape and position of quasimonoenergetic conversion electrons (<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>L</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub><mml:mtext>-</mml:mtext><mml:mn>32</mml:mn></mml:mrow></mml:math></inline-formula>) from <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Kr</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>83</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula> runs in <inline-formula><mml:math display="inline"><mml:msub><mml:mi>T</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math></inline-formula> to <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Kr</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>83</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula> runs without the carrier gas at 100 K <xref ref-type="bibr" rid="c47">[47]</xref>. We do not identify sizeable shifts (<inline-formula><mml:math display="inline"><mml:mo>&lt;</mml:mo><mml:mn>0.04</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula>) or broadening (<inline-formula><mml:math display="inline"><mml:mo>&lt;</mml:mo><mml:mn>0.08</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula>) of lines so that the contribution of plasma effects at <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:msub><mml:mi>d</mml:mi><mml:mi>exp</mml:mi></mml:msub></mml:math></inline-formula> to the systematic error budget in Table <xref ref-type="table" rid="t1">I</xref> can be neglected.</p><table-wrap id="t1" specific-use="style-1col"><object-id>I</object-id><object-id pub-id-type="doi">10.1103/PhysRevLett.123.221802.t1</object-id><label>TABLE I.</label><caption><p><inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1</mml:mn><mml:mi>σ</mml:mi></mml:mrow></mml:math></inline-formula> systematic uncertainties (<inline-formula><mml:math display="inline"><mml:msub><mml:mi>σ</mml:mi><mml:mrow><mml:mi>syst</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula>) for <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula> in <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mrow><mml:mi>eV</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, averaged over positive and negative errors, using the method of MC propagation.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="3"><oasis:colspec align="left" colname="col1" colsep="0" colwidth="43%"/><oasis:colspec align="center" colname="col2" colsep="0" colwidth="35%"/><oasis:colspec align="center" colname="col3" colsep="0" colwidth="25%"/><oasis:thead><oasis:row><oasis:entry align="left" valign="top">Effect</oasis:entry><oasis:entry align="center" valign="top">Relative uncertainty</oasis:entry><oasis:entry align="center" valign="top"><inline-formula><mml:math display="inline"><mml:mrow><mml:mi>σ</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:msubsup><mml:mrow><mml:mi>m</mml:mi></mml:mrow><mml:mrow><mml:mi>ν</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msubsup><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula> in <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mrow><mml:mi>eV</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry></oasis:row></oasis:thead><oasis:tbody><oasis:row rowsep="0"><oasis:entry>Source properties</oasis:entry><oasis:entry/><oasis:entry/></oasis:row><oasis:row rowsep="0"><oasis:entry><inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi><mml:mo>·</mml:mo><mml:mi>σ</mml:mi></mml:math></inline-formula></oasis:entry><oasis:entry>0.85%</oasis:entry><oasis:entry>0.05</oasis:entry></oasis:row><oasis:row rowsep="0"><oasis:entry>Energy loss <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>ϵ</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>δ</mml:mi><mml:mi mathvariant="normal">E</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry><oasis:entry><inline-formula><mml:math display="inline"><mml:mi mathvariant="script">O</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mn>1</mml:mn><mml:mo>%</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula></oasis:entry><oasis:entry>Negligible</oasis:entry></oasis:row><oasis:row rowsep="0"><oasis:entry>Beamline</oasis:entry><oasis:entry/><oasis:entry>0.05</oasis:entry></oasis:row><oasis:row rowsep="0"><oasis:entry><inline-formula><mml:math display="inline"><mml:msub><mml:mrow><mml:mi mathvariant="normal">B</mml:mi></mml:mrow><mml:mrow><mml:mi>WGTS</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula></oasis:entry><oasis:entry>2.5%</oasis:entry><oasis:entry/></oasis:row><oasis:row rowsep="0"><oasis:entry><inline-formula><mml:math display="inline"><mml:msub><mml:mrow><mml:mi mathvariant="normal">B</mml:mi></mml:mrow><mml:mi>min</mml:mi></mml:msub></mml:math></inline-formula></oasis:entry><oasis:entry>1%</oasis:entry><oasis:entry/></oasis:row><oasis:row rowsep="0"><oasis:entry><inline-formula><mml:math display="inline"><mml:msub><mml:mrow><mml:mi mathvariant="normal">B</mml:mi></mml:mrow><mml:mi>max</mml:mi></mml:msub></mml:math></inline-formula></oasis:entry><oasis:entry>0.2%</oasis:entry><oasis:entry/></oasis:row><oasis:row rowsep="0"><oasis:entry>Final state distribution</oasis:entry><oasis:entry><inline-formula><mml:math display="inline"><mml:mi mathvariant="script">O</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mn>1</mml:mn><mml:mo>%</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula></oasis:entry><oasis:entry>0.02</oasis:entry></oasis:row><oasis:row rowsep="0"><oasis:entry>Fluctuations in scan <inline-formula><mml:math display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula></oasis:entry><oasis:entry/><oasis:entry>0.05</oasis:entry></oasis:row><oasis:row rowsep="0"><oasis:entry>HV stacking</oasis:entry><oasis:entry>2 ppm</oasis:entry><oasis:entry/></oasis:row><oasis:row rowsep="0"><oasis:entry><inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi></mml:math></inline-formula> variation</oasis:entry><oasis:entry>0.8%</oasis:entry><oasis:entry/></oasis:row><oasis:row rowsep="0"><oasis:entry>Isotopologue fractions</oasis:entry><oasis:entry>0.2%</oasis:entry><oasis:entry/></oasis:row><oasis:row rowsep="0"><oasis:entry>Background</oasis:entry><oasis:entry/><oasis:entry/></oasis:row><oasis:row rowsep="0"><oasis:entry>Background slope</oasis:entry><oasis:entry>1.7%/keV</oasis:entry><oasis:entry>0.07</oasis:entry></oasis:row><oasis:row rowsep="0"><oasis:entry>Non-Poisson background</oasis:entry><oasis:entry>6.4%</oasis:entry><oasis:entry>0.30</oasis:entry></oasis:row><oasis:row rowsep="0"><oasis:entry>Total syst. uncertainty</oasis:entry><oasis:entry/><oasis:entry>0.32</oasis:entry></oasis:row></oasis:tbody></oasis:tgroup></oasis:table></table-wrap><p>The integral tritium <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay spectrum is scanned repeatedly in a range from [<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>E</mml:mi></mml:mrow><mml:mrow><mml:mn>0</mml:mn></mml:mrow></mml:msub><mml:mo>-</mml:mo><mml:mn>90</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>E</mml:mi></mml:mrow><mml:mrow><mml:mn>0</mml:mn></mml:mrow></mml:msub><mml:mo>+</mml:mo><mml:mn>50</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:mrow></mml:math></inline-formula>] by applying a set of nonequidistant HV settings to the inner electrode system. Each scan over this range takes a net time of about 2 h and is performed in alternating upward and downward directions to compensate for any time-dependent drift of the system to first order. At each HV set point, the transmitted electrons are counted over time intervals varying from 17 to 576 s with typical values of <inline-formula><mml:math display="inline"><mml:mo>∼</mml:mo><mml:mn>300</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mrow><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> for points close to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula>. When setting a new HV value, we make use of a custom-made postregulation system for voltage stabilization and elimination of high-frequency noise. At the same time, a custom-made HV divider <xref ref-type="bibr" rid="c48">[48]</xref> continuously monitors the retarding voltage with ppm precision.</p><p>To limit the influence of systematic uncertainties for this Letter, we analyze a scan range covering the region of 40 eV below <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> (22 HV set points) and 50 eV above (5 HV set points). The nonuniform measuring time distribution in this interval is shown in Fig. <xref ref-type="fig" rid="f3">3(c)</xref>. It maximizes the sensitivity for <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula> by focusing on the narrow region below <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula>, where the imprint of the neutrino mass on the spectrum is most pronounced <xref ref-type="bibr" rid="c20">[20]</xref>. Shorter time intervals with a set point 200 V below <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> are interspersed to monitor the source activity, in addition to other measures <xref ref-type="bibr" rid="c49">[49]</xref>.</p><fig id="f3"><object-id>3</object-id><object-id pub-id-type="doi">10.1103/PhysRevLett.123.221802.f3</object-id><label>FIG. 3.</label><caption><p>(a) Spectrum of electrons <inline-formula><mml:math display="inline"><mml:mi>R</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> over a 90 eV-wide interval from all 274 tritium scans and best-fit model <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> (line). The integral <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> decay spectrum extends up to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> on top of a flat background <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula>. Experimental data are stacked at the average value <inline-formula><mml:math display="inline"><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:msub><mml:mo stretchy="false">⟩</mml:mo><mml:mi>l</mml:mi></mml:msub></mml:math></inline-formula> of each HV set point and are displayed with <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1</mml:mn><mml:mi>σ</mml:mi></mml:mrow></mml:math></inline-formula> statistical uncertainties enlarged by a factor of 50. (b) Residuals of <inline-formula><mml:math display="inline"><mml:mi>R</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> relative to the <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1</mml:mn><mml:mi>σ</mml:mi></mml:mrow></mml:math></inline-formula> uncertainty band of the best fit model. (c) Integral measurement time distribution of all 27 HV set points.</p></caption><graphic xlink:href="e221802_3.eps"/></fig></sec><sec id="s5"><title specific-use="run-in">Data analysis.—</title><p>For each tritium scan with its 27 HV set points, we apply quality cuts to relevant slow-control parameters to select a data set with stable run conditions. This results in 274 scans with an overall scanning time of 521.7 h. We also define a list of 117 detector pixels (out of 148), which excludes those pixels that are noisy or shadowed by beam line instrumentation in the <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-electron path along the magnetic flux tube. For the digitized, calibrated and pile-up-corrected detector spectra, a broad region of interest (ROI) between 14 and 32 keV is defined. The ROI takes into account the detector energy resolution and its elevated potential (<inline-formula><mml:math display="inline"><mml:mrow><mml:mo>+</mml:mo><mml:mn>10</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>kV</mml:mi></mml:mrow></mml:math></inline-formula>) and allows us to include a large fraction of electrons backscattered at the detector in the narrow scan region close to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> resulting in a negligible contribution to the systematic uncertainty budget <xref ref-type="bibr" rid="c32">[32]</xref>.</p><p>The long-term stability of the scanning process is verified by fits to single scans to extract their effective <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay end points. The 274 fit values show no time-dependent behavior and follow a Gaussian distribution (<inline-formula><mml:math display="inline"><mml:mi>σ</mml:mi><mml:mo>=</mml:mo><mml:mn>0.25</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula>) around a mean value of <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>E</mml:mi></mml:mrow><mml:mrow><mml:mn>0</mml:mn></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:mn>18</mml:mn><mml:mtext> </mml:mtext><mml:mn>573.7</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:mrow></mml:math></inline-formula>. In view of this and the very good overall stability of the slow-control parameters for our data set, we merge the data of all 274 scans over all 117 pixels into one single 90-eV-wide spectrum, which is displayed in Fig. <xref ref-type="fig" rid="f3">3(a)</xref> in units of cps.</p><p>The underlying process corresponds to the “stacking” of events at the mean HV set points <inline-formula><mml:math display="inline"><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:msub><mml:mo stretchy="false">⟩</mml:mo><mml:mi>l</mml:mi></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mi>l</mml:mi><mml:mo>=</mml:mo><mml:mn>1</mml:mn><mml:mi>–</mml:mi><mml:mn>27</mml:mn></mml:math></inline-formula>). The small Gaussian spread (<inline-formula><mml:math display="inline"><mml:mrow><mml:mi>rms</mml:mi><mml:mo>=</mml:mo><mml:mn>34</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>mV</mml:mi></mml:mrow></mml:math></inline-formula>) of the actual HV value <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:msub><mml:mi>U</mml:mi><mml:mrow><mml:mi>l</mml:mi><mml:mo>,</mml:mo><mml:mi>k</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula> during a scan <inline-formula><mml:math display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula> relative to <inline-formula><mml:math display="inline"><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:msub><mml:mo stretchy="false">⟩</mml:mo><mml:mi>l</mml:mi></mml:msub></mml:math></inline-formula>, the average of all scans, is a minor systematic effect which is accounted for in the analysis. The resulting stacked integral spectrum, <inline-formula><mml:math display="inline"><mml:mrow><mml:mi mathvariant="normal">R</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula>, comprises <inline-formula><mml:math display="inline"><mml:mn>2.03</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mn>6</mml:mn></mml:msup></mml:math></inline-formula> events, with <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1.48</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mn>6</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>β</mml:mi></mml:mrow></mml:math></inline-formula>-decay electrons below <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> and a flat background ensemble of <inline-formula><mml:math display="inline"><mml:mn>0.55</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mn>6</mml:mn></mml:msup></mml:math></inline-formula> events in the 90 eV scan interval. This high-statistics data set allows us to show <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1</mml:mn><mml:mi>σ</mml:mi></mml:mrow></mml:math></inline-formula> error bars enlarged by a factor of 50 in Fig. <xref ref-type="fig" rid="f3">3</xref>.</p><p>The experimental spectrum is well described by our detailed model of the KATRIN response to <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay electrons and background. It contains four free parameters: the signal amplitude <inline-formula><mml:math display="inline"><mml:msub><mml:mi>A</mml:mi><mml:mi>s</mml:mi></mml:msub></mml:math></inline-formula>, the effective <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay end point <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula>, the background rate <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula>, and the neutrino mass square <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula>. We leave <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:msub><mml:mi>A</mml:mi><mml:mi>s</mml:mi></mml:msub></mml:math></inline-formula> unconstrained, which is equivalent to a “shape-only” fit. The goodness-of-fit is illustrated in Fig. <xref ref-type="fig" rid="f3">3(b)</xref> from the scatter of residuals around the error band of the model.</p><p>The four-parameter fit procedure over the averaged HV set points <inline-formula><mml:math display="inline"><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:msub><mml:mo stretchy="false">⟩</mml:mo><mml:mi>l</mml:mi></mml:msub></mml:math></inline-formula> compares the experimental spectrum <inline-formula><mml:math display="inline"><mml:mrow><mml:mi mathvariant="normal">R</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula> to the model <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula>. The latter is the convolution of the differential <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-electron spectrum <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>β</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula> with the calculated response function <inline-formula><mml:math display="inline"><mml:msub><mml:mi>f</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula>, with an added energy-independent background rate <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula> <disp-formula id="d1"><mml:math display="block"><mml:mrow><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo><mml:mo>=</mml:mo><mml:msub><mml:mrow><mml:mi>A</mml:mi></mml:mrow><mml:mrow><mml:mi>s</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mrow><mml:mi>N</mml:mi></mml:mrow><mml:mrow><mml:mi>T</mml:mi></mml:mrow></mml:msub><mml:mo>∫</mml:mo><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>β</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo stretchy="false">)</mml:mo><mml:msub><mml:mrow><mml:mi>f</mml:mi></mml:mrow><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo><mml:mi>d</mml:mi><mml:mi>E</mml:mi><mml:mo>+</mml:mo><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>bg</mml:mi></mml:mrow></mml:msub><mml:mo>.</mml:mo><mml:mspace linebreak="goodbreak"/><mml:malignmark/></mml:mrow></mml:math><label>(1)</label></disp-formula>Here, <inline-formula><mml:math display="inline"><mml:msub><mml:mi>N</mml:mi><mml:mi>T</mml:mi></mml:msub></mml:math></inline-formula> denotes the calculated number of tritium atoms in the source multiplied with the accepted solid angle of the setup <inline-formula><mml:math display="inline"><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi mathvariant="normal">Ω</mml:mi><mml:mo stretchy="false">/</mml:mo><mml:mn>4</mml:mn><mml:mi>π</mml:mi><mml:mo>=</mml:mo><mml:mo stretchy="false">(</mml:mo><mml:mn>1</mml:mn><mml:mo>-</mml:mo><mml:mi>cos</mml:mi><mml:msub><mml:mi>θ</mml:mi><mml:mi>max</mml:mi></mml:msub><mml:mo stretchy="false">)</mml:mo><mml:mo stretchy="false">/</mml:mo><mml:mn>2</mml:mn></mml:math></inline-formula> and the detector efficiency [<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>θ</mml:mi></mml:mrow><mml:mrow><mml:mi>max</mml:mi></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:mi>arcsin</mml:mi><mml:msqrt><mml:mrow><mml:mo stretchy="false">(</mml:mo><mml:msub><mml:mrow><mml:mi>B</mml:mi></mml:mrow><mml:mrow><mml:mi>WGTS</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">/</mml:mo><mml:msub><mml:mrow><mml:mi>B</mml:mi></mml:mrow><mml:mrow><mml:mi>max</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:msqrt><mml:mo>=</mml:mo><mml:mn>50.4</mml:mn><mml:mi>°</mml:mi></mml:mrow></mml:math></inline-formula>], its uncertainty is absorbed by the fit parameter <inline-formula><mml:math display="inline"><mml:msub><mml:mi>A</mml:mi><mml:mi>s</mml:mi></mml:msub></mml:math></inline-formula>.</p><p>The electron spectrum <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>β</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula> from the superallowed <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> decay of molecular tritium is calculated using Fermi’s Golden Rule <disp-formula id="d2"><mml:math display="block"><mml:mrow><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>β</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo stretchy="false">)</mml:mo><mml:mo id="d2a1">=</mml:mo><mml:mfrac><mml:mrow><mml:msubsup><mml:mrow><mml:mi>G</mml:mi></mml:mrow><mml:mrow><mml:mi>F</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msubsup><mml:mo>·</mml:mo><mml:msup><mml:mrow><mml:mi>cos</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup><mml:msub><mml:mrow><mml:mi mathvariant="normal">Θ</mml:mi></mml:mrow><mml:mrow><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:mn>2</mml:mn><mml:msup><mml:mrow><mml:mi>π</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:mfrac><mml:mo stretchy="false">|</mml:mo><mml:msubsup><mml:mrow><mml:mi>M</mml:mi></mml:mrow><mml:mrow><mml:mi>nucl</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msubsup><mml:mo stretchy="false">|</mml:mo><mml:mi>F</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>,</mml:mo><mml:msup><mml:mrow><mml:mi>Z</mml:mi></mml:mrow><mml:mrow><mml:mo>′</mml:mo></mml:mrow></mml:msup><mml:mo stretchy="false">)</mml:mo><mml:mspace linebreak="newline"/><mml:mo indentalign="id" indentshift="1em" indenttarget="d2a1">⁢</mml:mo><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>+</mml:mo><mml:msub><mml:mrow><mml:mi>m</mml:mi></mml:mrow><mml:mrow><mml:mi mathvariant="normal">e</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">)</mml:mo><mml:msqrt><mml:mrow><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>+</mml:mo><mml:msub><mml:mrow><mml:mi>m</mml:mi></mml:mrow><mml:mrow><mml:mi mathvariant="normal">e</mml:mi></mml:mrow></mml:msub><mml:msup><mml:mrow><mml:mo stretchy="false">)</mml:mo></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup><mml:mo>-</mml:mo><mml:msubsup><mml:mrow><mml:mi>m</mml:mi></mml:mrow><mml:mrow><mml:mi mathvariant="normal">e</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msubsup></mml:mrow></mml:msqrt><mml:mspace linebreak="newline"/><mml:mo indentalign="id" indentshift="1em" indenttarget="d2a1">⁢</mml:mo><mml:munder><mml:mrow><mml:mo>∑</mml:mo></mml:mrow><mml:mrow><mml:mi mathvariant="normal">j</mml:mi></mml:mrow></mml:munder><mml:msub><mml:mrow><mml:mi>ζ</mml:mi></mml:mrow><mml:mrow><mml:mi>j</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mrow><mml:mi>ϵ</mml:mi></mml:mrow><mml:mrow><mml:mi>j</mml:mi></mml:mrow></mml:msub><mml:msqrt><mml:mrow><mml:msubsup><mml:mrow><mml:mi>ϵ</mml:mi></mml:mrow><mml:mrow><mml:mi>j</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msubsup><mml:mo>-</mml:mo><mml:msubsup><mml:mrow><mml:mi>m</mml:mi></mml:mrow><mml:mrow><mml:mi>ν</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msubsup></mml:mrow></mml:msqrt><mml:mi mathvariant="normal">Θ</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:msub><mml:mrow><mml:mi>ϵ</mml:mi></mml:mrow><mml:mrow><mml:mi>j</mml:mi></mml:mrow></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mrow><mml:mi>m</mml:mi></mml:mrow><mml:mrow><mml:mi>ν</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">)</mml:mo><mml:mo>,</mml:mo></mml:mrow></mml:math><label>(2)</label></disp-formula>with the square of the energy-independent nuclear matrix element <inline-formula><mml:math display="inline"><mml:mo stretchy="false">|</mml:mo><mml:msubsup><mml:mi>M</mml:mi><mml:mrow><mml:mi>nucl</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msubsup><mml:mo stretchy="false">|</mml:mo></mml:math></inline-formula>, the Fermi constant <inline-formula><mml:math display="inline"><mml:msub><mml:mi>G</mml:mi><mml:mi>F</mml:mi></mml:msub></mml:math></inline-formula>, the Cabibbo angle <inline-formula><mml:math display="inline"><mml:msub><mml:mi mathvariant="normal">Θ</mml:mi><mml:mi>C</mml:mi></mml:msub></mml:math></inline-formula>, the electron mass <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>e</mml:mi></mml:msub></mml:math></inline-formula>, the Fermi function <inline-formula><mml:math display="inline"><mml:mi>F</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>,</mml:mo><mml:msup><mml:mi>Z</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>=</mml:mo><mml:mn>2</mml:mn><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula>, and the neutrino energy <inline-formula><mml:math display="inline"><mml:msub><mml:mi>ϵ</mml:mi><mml:mi>j</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub><mml:mo>-</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:msub><mml:mi>V</mml:mi><mml:mi>j</mml:mi></mml:msub></mml:math></inline-formula>. In addition, our calculations incorporate radiative corrections (for details, see <xref ref-type="bibr" rid="c12 c20">[12,20]</xref>), and we account for thermal Doppler broadening at 30 K.</p><p>When calculating <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>β</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula>, we sum over a final-state distribution (FSD) which is given by the probabilities <inline-formula><mml:math display="inline"><mml:msub><mml:mi>ζ</mml:mi><mml:mi>j</mml:mi></mml:msub></mml:math></inline-formula> with which the daughter ion <inline-formula><mml:math display="inline"><mml:mrow><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>He</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow><mml:mrow><mml:msup><mml:mrow><mml:mi>T</mml:mi></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:mrow></mml:math></inline-formula> is left in a molecular (i.e., a rotational, vibrational, and electronic) state with excitation energy <inline-formula><mml:math display="inline"><mml:msub><mml:mi>V</mml:mi><mml:mi>j</mml:mi></mml:msub></mml:math></inline-formula>. For this analysis, we first confirm the most recent theoretical FSD calculations <xref ref-type="bibr" rid="c50 c51">[50,51]</xref> using new codes for solving the electronic and rovibrational problems within the Born-Oppenheimer approximation. We then refine the FSD by adopting a more efficient treatment of the rovibrational part and an update of other kinematics-related quantities, such as molecular masses, as well as recoil parameters (momenta and kinetic energy shifts). Most importantly, we treat all isotopologues (<inline-formula><mml:math display="inline"><mml:msub><mml:mi>T</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math></inline-formula>, HT, and DT) in a consistent way with initial angular momenta distributions <inline-formula><mml:math display="inline"><mml:msub><mml:mi>J</mml:mi><mml:mi>κ</mml:mi></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mi>κ</mml:mi><mml:mo>=</mml:mo><mml:mn>0</mml:mn><mml:mo>,</mml:mo><mml:mo>…</mml:mo><mml:mo>,</mml:mo><mml:mn>3</mml:mn></mml:math></inline-formula>) at 30 K for the electronic bound states <inline-formula><mml:math display="inline"><mml:mi>n</mml:mi><mml:mo>=</mml:mo><mml:mn>1</mml:mn><mml:mo>,</mml:mo><mml:mo>…</mml:mo><mml:mo>,</mml:mo><mml:mn>6</mml:mn></mml:math></inline-formula>. The FSD includes higher excitation energies up to the continuum based on <xref ref-type="bibr" rid="c50">[50]</xref>, but their contribution to our analysis interval [<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>E</mml:mi></mml:mrow><mml:mrow><mml:mn>0</mml:mn></mml:mrow></mml:msub><mml:mo>-</mml:mo><mml:mn>40</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:mrow></mml:math></inline-formula>] is at an overall level of <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mn>4</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> only. Accordingly, the FSD uncertainties in our narrow analysis interval of 40 eV below <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> only contribute at the level of <inline-formula><mml:math display="inline"><mml:mn>0.02</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:msup><mml:mi>eV</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:math></inline-formula> to the total systematics budget on <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula> (see Table <xref ref-type="table" rid="t1">I</xref>).</p><p>The response function <inline-formula><mml:math display="inline"><mml:msub><mml:mi>f</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> used in the analysis is shown as the red curve in Fig. <xref ref-type="fig" rid="f2">2</xref> (top). It corresponds to <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay electrons born with energies close to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> and emitted isotropically up to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>θ</mml:mi><mml:mi>max</mml:mi></mml:msub></mml:math></inline-formula> in the source gas. Compared to the <inline-formula><mml:math display="inline"><mml:mi>e</mml:mi></mml:math></inline-formula>-gun beam, they possess a different distribution of energy losses due to their broader range of pitch angles <inline-formula><mml:math display="inline"><mml:mi>θ</mml:mi></mml:math></inline-formula> and the varying amount of source gas (<inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi></mml:math></inline-formula>) they traverse. These processes are studied on the basis of gas dynamical simulations <xref ref-type="bibr" rid="c52">[52]</xref> which yield an approximately triangular-shaped longitudinal source profile.</p><p>After modeling the energy loss of <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay electrons through the source by making use of <inline-formula><mml:math display="inline"><mml:mi>ρ</mml:mi><mml:mi>d</mml:mi><mml:mo>·</mml:mo><mml:mi>σ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>ϵ</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>δ</mml:mi><mml:mi>E</mml:mi><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula>, their subsequent propagation is tracked by the <sc>kassiopeia</sc> simulation software <xref ref-type="bibr" rid="c53">[53]</xref>. It incorporates a detailed beam line model which takes account of the small radial inhomogeneities of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>B</mml:mi><mml:mi>min</mml:mi></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mi>q</mml:mi><mml:mi>U</mml:mi></mml:math></inline-formula> at the analyzing plane. The full model provides the detailed shape of <inline-formula><mml:math display="inline"><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>E</mml:mi></mml:math></inline-formula> and the distribution of electron pitch angles up to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>θ</mml:mi><mml:mi>max</mml:mi></mml:msub></mml:math></inline-formula> from the parameters of the magnetic field triplet (<inline-formula><mml:math display="inline"><mml:msub><mml:mi>B</mml:mi><mml:mrow><mml:mi>WGTS</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula>, <inline-formula><mml:math display="inline"><mml:msub><mml:mi>B</mml:mi><mml:mi>min</mml:mi></mml:msub></mml:math></inline-formula>, <inline-formula><mml:math display="inline"><mml:msub><mml:mi>B</mml:mi><mml:mi>max</mml:mi></mml:msub></mml:math></inline-formula>).</p><p>The energy-independent part of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula>, <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula>, comes from a fit of the spectrum <inline-formula><mml:math display="inline"><mml:mrow><mml:mi mathvariant="normal">R</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:mrow></mml:math></inline-formula> over our 90 eV scan range. The fit value <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mo stretchy="false">(</mml:mo><mml:mn>0.293</mml:mn><mml:mo>±</mml:mo><mml:mn>0.001</mml:mn><mml:mo stretchy="false">)</mml:mo><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>cps</mml:mi></mml:math></inline-formula> is largely constrained by the 5 HV set points above <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> and agrees with data from independent background runs taken with an empty source before the tritium measurements.</p><p>The resulting model, <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula>, is then fitted to <inline-formula><mml:math display="inline"><mml:mi>R</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula>. To ensure that this proceeds without bias, we employ a twofold “blinding” scheme. The first blinding step leaves the data untouched, but a modification is applied during the building of the model <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula>. The FSD part describing rovibrational excitations of the electronic ground state is replaced with a Gaussian distribution with parameters not accessible to the analysis at first. As a result, fits with the blinded FSD do not reveal the unbiased value of <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula>. The “true” FSD is revealed only at the last step (“unblinding”) after having fixed all model inputs and systematic uncertainties.</p><p>The second measure to mitigate biasing is to perform the full analysis, including parameter fitting, using Monte Carlo–based (MC) data sets first, before turning to the experimental data. For each experimental scan <inline-formula><mml:math display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula>, we generate a “MC twin,” <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:msub><mml:mrow><mml:mo stretchy="false">)</mml:mo></mml:mrow><mml:mrow><mml:mi>k</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, from its averaged slow-control parameters to procure <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mi>β</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:msub><mml:mrow><mml:mo stretchy="false">)</mml:mo></mml:mrow><mml:mrow><mml:mi>k</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math display="inline"><mml:msub><mml:mi>f</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mi>E</mml:mi><mml:mo>-</mml:mo><mml:mspace linebreak="goodbreak"/><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:msub><mml:mo stretchy="false">)</mml:mo><mml:mi>k</mml:mi></mml:msub></mml:math></inline-formula>, and <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>bg</mml:mi><mml:mo>,</mml:mo><mml:mi>k</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula>. Analysis of MC twins allows us to verify the accuracy of our parameter inference by recovering the correct input MC values for <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula>. This approach is also used to assess statistical (<inline-formula><mml:math display="inline"><mml:msub><mml:mi>σ</mml:mi><mml:mrow><mml:mi>stat</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula>) and systematic (<inline-formula><mml:math display="inline"><mml:msub><mml:mi>σ</mml:mi><mml:mrow><mml:mi>syst</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula>) uncertainties and to compute our expected sensitivity.</p><p>In the following, we report on the results of two independent analyses with different strategies to propagate systematic uncertainties: the “Covariance Matrix” and the “MC propagation” approaches.</p><p>In the covariance method, we fit the experimental spectrum <inline-formula><mml:math display="inline"><mml:mi>R</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> with the model <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> by minimizing the standard <inline-formula><mml:math display="inline"><mml:msup><mml:mi>χ</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:math></inline-formula> estimator. To propagate the systematic uncertainties, a covariance matrix is computed after performing <inline-formula><mml:math display="inline"><mml:mi>O</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mn>4</mml:mn></mml:msup><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> simulations of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula>, while varying the relevant parameters for each calculation according to the likelihood given by their uncertainties <xref ref-type="bibr" rid="c35 c54 c55">[35,54,55]</xref>. The resulting systematic uncertainties agree with the values shown in Table <xref ref-type="table" rid="t1">I</xref>, which is based on the second approach. The sum of all matrices encodes the total uncertainties of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> and their HV set point dependent correlations. The <inline-formula><mml:math display="inline"><mml:msup><mml:mi>χ</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:math></inline-formula> estimator is then minimized to determine the four best-fit parameters, and the shape of <inline-formula><mml:math display="inline"><mml:msup><mml:mi>χ</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:math></inline-formula> function is used to infer the uncertainties. The results of this fit are displayed in Fig. <xref ref-type="fig" rid="f3">3</xref>. We obtain a goodness-of-fit of <inline-formula><mml:math display="inline"><mml:msup><mml:mi>χ</mml:mi><mml:mn>2</mml:mn></mml:msup><mml:mo>=</mml:mo><mml:mn>21.4</mml:mn></mml:math></inline-formula> for 23 d.o.f., corresponding to a <inline-formula><mml:math display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula> value of 0.56.</p><p>The MC-propagation approach is a hybrid Bayesian-frequentist method, adapted from Refs. <xref ref-type="bibr" rid="c56 c57 c58">[56–58]</xref>. We fit the experimental spectrum <inline-formula><mml:math display="inline"><mml:mi>R</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> with the model <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi>calc</mml:mi></mml:mrow></mml:msub><mml:mo stretchy="false">(</mml:mo><mml:mo stretchy="false">⟨</mml:mo><mml:mi>q</mml:mi><mml:mi>U</mml:mi><mml:mo stretchy="false">⟩</mml:mo><mml:mo stretchy="false">)</mml:mo></mml:math></inline-formula> by minimizing the negative Poisson-likelihood function. The goodness-of-fit of <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo><mml:mn>2</mml:mn><mml:mi>ln</mml:mi><mml:mi mathvariant="script">L</mml:mi><mml:mo>=</mml:mo><mml:mn>23.3</mml:mn></mml:math></inline-formula> for 23 d.o.f. corresponds to a <inline-formula><mml:math display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula> value of 0.44. To propagate the systematic uncertainties, we repeat the fit <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mn>5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> times, while varying the relevant parameters in each fit according to their uncertainties given in column 2 of Table <xref ref-type="table" rid="t1">I</xref>.</p><p>We report the <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1</mml:mn><mml:mi>σ</mml:mi></mml:mrow></mml:math></inline-formula> width of the fit parameters as their systematic uncertainty in the third column of Table <xref ref-type="table" rid="t1">I</xref>. In order to simultaneously treat statistical and all systematic uncertainties, each of the <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mrow><mml:mn>10</mml:mn></mml:mrow><mml:mrow><mml:mn>5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> fits is performed on a statistically fluctuated MC copy of the true data set, leading to the distributions of <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> shown in Fig. <xref ref-type="fig" rid="f4">4</xref>. The strong correlation (0.97) between the two parameters is an expected feature in kinematic studies of <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula> decay <xref ref-type="bibr" rid="c11 c12">[11,12]</xref>. The final-best fit is given by the mode of the fit-parameter distributions, and the <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1</mml:mn><mml:mi>σ</mml:mi></mml:mrow></mml:math></inline-formula> total error is determined by integrating the distributions up to 16% from either side.</p><fig id="f4"><object-id>4</object-id><object-id pub-id-type="doi">10.1103/PhysRevLett.123.221802.f4</object-id><label>FIG. 4.</label><caption><p>Scatter plot of fit values for the mass square <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula> and the effective <inline-formula><mml:math display="inline"><mml:mi>β</mml:mi></mml:math></inline-formula>-decay end point <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> together with <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1</mml:mn><mml:mi>σ</mml:mi></mml:mrow></mml:math></inline-formula> (black) and <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>2</mml:mn><mml:mi>σ</mml:mi></mml:mrow></mml:math></inline-formula> (blue) error contours around the best fit point (cross). It follows from a large set of pseudoexperiments emulating our experimental data set and its statistical and systematical uncertainties.</p></caption><graphic xlink:href="e221802_4.eps"/></fig></sec><sec id="s6"><title specific-use="run-in">Results.—</title><p>The two independent methods agree to within a few percent of the total uncertainty. As best fit value for the neutrino mass, we find <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mrow><mml:mi>m</mml:mi></mml:mrow><mml:mrow><mml:mi>ν</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msubsup><mml:mo>=</mml:mo><mml:mo stretchy="false">(</mml:mo><mml:mo>-</mml:mo><mml:msubsup><mml:mrow><mml:mn>1.0</mml:mn></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mn>1.1</mml:mn></mml:mrow><mml:mrow><mml:mo>+</mml:mo><mml:mn>0.9</mml:mn></mml:mrow></mml:msubsup><mml:mo stretchy="false">)</mml:mo><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:msup><mml:mrow><mml:mi>eV</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. This best fit result corresponds to a <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>1</mml:mn><mml:mi>σ</mml:mi></mml:mrow></mml:math></inline-formula> statistical fluctuation to negative values of <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula> possessing a <inline-formula><mml:math display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula> value of 0.16.</p><p>The total uncertainty budget of <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula> is largely dominated by <inline-formula><mml:math display="inline"><mml:msub><mml:mi>σ</mml:mi><mml:mrow><mml:mi>stat</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mn>0.97</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:msup><mml:mi>eV</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:math></inline-formula>) as compared to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>σ</mml:mi><mml:mrow><mml:mi>syst</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mn>0.32</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:msup><mml:mi>eV</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:math></inline-formula>). As displayed in Table <xref ref-type="table" rid="t1">I</xref>, the dominant contributions to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>σ</mml:mi><mml:mrow><mml:mi>syst</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula> are found to be the non-Poissonian background from radon and the uncertainty on the background slope, which is constrained from the wide-energy integral scans of the earlier “first tritium” data <xref ref-type="bibr" rid="c35">[35]</xref>. Uncertainties of the column density, energy-loss function, final-state distribution, and magnetic fields play a minor role in the budget of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>σ</mml:mi><mml:mrow><mml:mi>syst</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula>. Likewise, the uncertainties induced via fluctuations of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>ϵ</mml:mi><mml:mi>T</mml:mi></mml:msub></mml:math></inline-formula> and HV parameters during a scan are negligibly small compared to <inline-formula><mml:math display="inline"><mml:msub><mml:mi>σ</mml:mi><mml:mrow><mml:mi>stat</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula>. The statistical (systematic) uncertainty of our first result on <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula> is smaller by a factor of 2 (6) compared to the final results of Troitsk and Mainz <xref ref-type="bibr" rid="c24 c25">[24,25]</xref>.</p><p>The methods of Lokhov and Tkachov (LT) <xref ref-type="bibr" rid="c59">[59]</xref> and of Feldman and Cousins (FC) <xref ref-type="bibr" rid="c60">[60]</xref> are then used to calculate the upper limit on <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub></mml:math></inline-formula>. Both procedures avoid empty confidence intervals for nonphysical negative best-fit estimates of <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula>. For this first result, we follow the LT method. For a statistical fluctuation into the nonphysical region the method returns a confidence belt that coincides with the experimental sensitivity and avoids a shrinking upper limit for more negative values of <inline-formula><mml:math display="inline"><mml:msubsup><mml:mi>m</mml:mi><mml:mi>ν</mml:mi><mml:mn>2</mml:mn></mml:msubsup></mml:math></inline-formula>. Using the LT construction, we derive an upper limit of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub><mml:mo>&lt;</mml:mo><mml:mn>1.1</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula> (90% C.L.) as the central result of this Letter. By construction, it is identical to the expected sensitivity. For completeness, we also note the FC upper limits <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub><mml:mo>&lt;</mml:mo><mml:mn>0.8</mml:mn><mml:mo stretchy="false">(</mml:mo><mml:mn>0.9</mml:mn><mml:mo stretchy="false">)</mml:mo><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula> at 90% (95%) C.L.</p><p>For the effective end point, our two analysis methods both obtain the best-fit value <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>E</mml:mi></mml:mrow><mml:mrow><mml:mn>0</mml:mn></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:mo stretchy="false">(</mml:mo><mml:mn>18</mml:mn><mml:mtext> </mml:mtext><mml:mn>573.7</mml:mn><mml:mo>±</mml:mo><mml:mn>0.1</mml:mn><mml:mo stretchy="false">)</mml:mo><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:mrow></mml:math></inline-formula> (see Fig. <xref ref-type="fig" rid="f4">4</xref>). At this level of precision, a consistency check on the energy scale of KATRIN can be performed by comparing our experimental <inline-formula><mml:math display="inline"><mml:mi>Q</mml:mi></mml:math></inline-formula> value for molecular tritium with that based on measurements of the <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>He</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:mmultiscripts><mml:mtext>-</mml:mtext><mml:mmultiscripts><mml:mrow><mml:mi mathvariant="normal">H</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula> atomic mass difference <xref ref-type="bibr" rid="c61">[61]</xref>. Our result for the <inline-formula><mml:math display="inline"><mml:mi>Q</mml:mi></mml:math></inline-formula> value of <inline-formula><mml:math display="inline"><mml:mo stretchy="false">(</mml:mo><mml:mn>18</mml:mn><mml:mn>575.2</mml:mn><mml:mo>±</mml:mo><mml:mn>0.5</mml:mn><mml:mo stretchy="false">)</mml:mo><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula> is obtained from our best-fit value for <inline-formula><mml:math display="inline"><mml:msub><mml:mi>E</mml:mi><mml:mn>0</mml:mn></mml:msub></mml:math></inline-formula> by adding the center-of-mass molecular recoil of <inline-formula><mml:math display="inline"><mml:msub><mml:mi>T</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math></inline-formula> (1.72 eV) <xref ref-type="bibr" rid="c11">[11]</xref>, as well as the relative offset (<inline-formula><mml:math display="inline"><mml:mo>-</mml:mo><mml:mn>0.2</mml:mn><mml:mo>±</mml:mo><mml:mn>0.5</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula>) of the source potential to the work function of the inner electrode. The calculated <inline-formula><mml:math display="inline"><mml:mi>Q</mml:mi></mml:math></inline-formula> value from the <inline-formula><mml:math display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>He</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:mmultiscripts><mml:mtext>-</mml:mtext><mml:mmultiscripts><mml:mrow><mml:mi mathvariant="normal">H</mml:mi></mml:mrow><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math></inline-formula> atomic mass difference is <inline-formula><mml:math display="inline"><mml:mo stretchy="false">(</mml:mo><mml:mn>18</mml:mn><mml:mn>575.72</mml:mn><mml:mo>±</mml:mo><mml:mn>0.07</mml:mn><mml:mo stretchy="false">)</mml:mo><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula> when accounting for the different binding energies and kinematic variables of atomic and molecular tritium <xref ref-type="bibr" rid="c11">[11]</xref>. The consistency of both <inline-formula><mml:math display="inline"><mml:mi>Q</mml:mi></mml:math></inline-formula> values underlines the robustness of the energy scale in our scanning process of molecular tritium.</p></sec><sec id="s7"><title specific-use="run-in">Conclusion and outlook.—</title><p>The reported upper limit <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub><mml:mo>&lt;</mml:mo><mml:mn>1.1</mml:mn><mml:mtext> </mml:mtext><mml:mtext> </mml:mtext><mml:mi>eV</mml:mi></mml:math></inline-formula> (90% C.L.) improves upon previous results <xref ref-type="bibr" rid="c24 c25">[24,25]</xref> by almost a factor of 2 after a measuring period of only four weeks while operating at reduced column density. It is based on a purely kinematic method. As such, it has implications for both particle physics and cosmology. For the former, it narrows down the allowed range of quasidegenerate neutrino mass models by a direct method. For the latter, this model-independent limit can be used as laboratory-based input for studies of structure evolution in <inline-formula><mml:math display="inline"><mml:mi mathvariant="normal">Λ</mml:mi><mml:mi>CDM</mml:mi></mml:math></inline-formula> and other cosmological models.</p><p>Our result shows the potential of KATRIN to probe <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub></mml:math></inline-formula> by a direct kinematic method. After 1000 days of data taking at nominal column density and further reductions of systematics and <inline-formula><mml:math display="inline"><mml:msub><mml:mi>R</mml:mi><mml:mi>bg</mml:mi></mml:msub></mml:math></inline-formula>, we will reach a sensitivity of 0.2 eV (90% C.L.) on <inline-formula><mml:math display="inline"><mml:msub><mml:mi>m</mml:mi><mml:mi>ν</mml:mi></mml:msub></mml:math></inline-formula>, augmented by searches for physics beyond the SM, such as for sterile neutrino admixtures with masses from the eV to the keV scale.</p></sec></body><back><ack><p>We acknowledge the support of the Helmholtz Association, Ministry for Education and Research BMBF (Grants No. 5A17PDA, No. 05A17PM3, No. 05A17PX3, No. 05A17VK2, and No. 05A17WO3), Helmholtz Alliance for Astroparticle Physics (HAP), Helmholtz Young Investigator Group (Grant No. VH-NG-1055), Max Planck Research Group (MaxPlanck@TUM), and Deutsche Forschungsgemeinschaft DFG (Research Training Groups Grants No. GRK 1694 and No. GRK 2149, and Graduate School Grant No. GSC 1085—KSETA) in Germany; Ministry of Education, Youth and Sport (Grants No. CANAM-LM2011019, and No. LTT19005) in the Czech Republic; and the United States Department of Energy through Grants No. DE-FG02-97ER41020, No. DE-FG02-94ER40818, No. DE-SC0004036, No. DE-FG02-97ER41033, No. DE-FG02-97ER41041, No. DE-AC02-05CH11231, No. DE-SC0011091, and No. DE-SC0019304, and the National Energy Research Scientific Computing Center.</p></ack><ref-list><ref id="c1"><label>[1]</label><mixed-citation publication-type="journal"><object-id>1</object-id><person-group person-group-type="author"><string-name>Y. 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